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Description
| - Electronic structure calculations combining the local-density approximation with an exact diagonalization of the Anderson impurity model show an intermediate 5f5-5f6-valence ground state and delocalization of the 5f5 multiplet of the Pu atom 5f shell in PuCoIn5, PuCoGa5, and δ-Pu. The 5f local magnetic moment is compensated by a moment formed in the surrounding cloud of conduction electrons. For PuCoGa5 and δ-Pu the compensation is complete, and the Anderson impurity ground state is a singlet. For PuCoIn5 the compensation is partial, and the Pu ground state is magnetic. We suggest that the unconventional d-wave superconductivity is likely mediated by the 5f-state antiferromagnetic fluctuations in PuCoIn5 and by valence fluctuations in PuCoGa5.
- Electronic structure calculations combining the local-density approximation with an exact diagonalization of the Anderson impurity model show an intermediate 5f5-5f6-valence ground state and delocalization of the 5f5 multiplet of the Pu atom 5f shell in PuCoIn5, PuCoGa5, and δ-Pu. The 5f local magnetic moment is compensated by a moment formed in the surrounding cloud of conduction electrons. For PuCoGa5 and δ-Pu the compensation is complete, and the Anderson impurity ground state is a singlet. For PuCoIn5 the compensation is partial, and the Pu ground state is magnetic. We suggest that the unconventional d-wave superconductivity is likely mediated by the 5f-state antiferromagnetic fluctuations in PuCoIn5 and by valence fluctuations in PuCoGa5. (en)
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Title
| - Unified character of correlation effects in unconventional Pu-based superconductors and δ-Pu
- Unified character of correlation effects in unconventional Pu-based superconductors and δ-Pu (en)
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skos:prefLabel
| - Unified character of correlation effects in unconventional Pu-based superconductors and δ-Pu
- Unified character of correlation effects in unconventional Pu-based superconductors and δ-Pu (en)
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skos:notation
| - RIV/68378271:_____/13:00397088!RIV14-GA0-68378271
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http://linked.open...avai/predkladatel
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http://linked.open...avai/riv/aktivita
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http://linked.open...avai/riv/aktivity
| - I, P(GAP204/10/0330), P(IAA100100912)
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http://linked.open...iv/cisloPeriodika
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http://linked.open...vai/riv/dodaniDat
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http://linked.open...aciTvurceVysledku
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http://linked.open.../riv/druhVysledku
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http://linked.open...iv/duvernostUdaju
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http://linked.open...titaPredkladatele
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http://linked.open...dnocenehoVysledku
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http://linked.open...ai/riv/idVysledku
| - RIV/68378271:_____/13:00397088
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http://linked.open...riv/jazykVysledku
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http://linked.open.../riv/klicovaSlova
| - superconductivity; magnetism; plutonium (en)
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http://linked.open.../riv/klicoveSlovo
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http://linked.open...odStatuVydavatele
| - US - Spojené státy americké
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http://linked.open...ontrolniKodProRIV
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http://linked.open...i/riv/nazevZdroje
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http://linked.open...in/vavai/riv/obor
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http://linked.open...ichTvurcuVysledku
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http://linked.open...cetTvurcuVysledku
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http://linked.open...vavai/riv/projekt
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http://linked.open...UplatneniVysledku
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http://linked.open...v/svazekPeriodika
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http://linked.open...iv/tvurceVysledku
| - Kolorenč, Jindřich
- Oppeneer, P. M.
- Shick, Alexander
- Caciuffo, R.
- Lichtenstein, A. I.
- Rusz, Ján
- Katsnelson, M. I.
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http://linked.open...ain/vavai/riv/wos
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issn
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number of pages
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http://bibframe.org/vocab/doi
| - 10.1103/PhysRevB.87.020505
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