About: Ferroelectric phase transition in polycrystalline KTaO3 thin film revealed by terahertz spectroscopy     Goto   Sponge   NotDistinct   Permalink

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  • KTaO3 single crystal is an archetypal incipient ferroelectric in which a long-range ferroelectric order does not establish at low temperatures owing to quantum fluctuations. We report on a strong evidence of the ferroelectric phase transition near 60 K revealed by terahertz spectroscopy and microwave permittivity measurements of a polycrystalline KTaO3 thin film on (0001) sapphire substrate prepared by chemical solution deposition. The soft mode behavior is clearly observed in the terahertz (THz) spectra with a minimum frequency at 60 K. At the same temperature microwave permittivity maximum appears. The THz spectra strongly resemble that of strained epitaxial SrTiO3/DyScO3 films: the ferroelectric soft mode is linearly coupled to a central peak which is silent in the paraelectric phase and it becomes coupled to the polarization below the ferroelectric transition temperature with a progressively increasing bare strength.
  • KTaO3 single crystal is an archetypal incipient ferroelectric in which a long-range ferroelectric order does not establish at low temperatures owing to quantum fluctuations. We report on a strong evidence of the ferroelectric phase transition near 60 K revealed by terahertz spectroscopy and microwave permittivity measurements of a polycrystalline KTaO3 thin film on (0001) sapphire substrate prepared by chemical solution deposition. The soft mode behavior is clearly observed in the terahertz (THz) spectra with a minimum frequency at 60 K. At the same temperature microwave permittivity maximum appears. The THz spectra strongly resemble that of strained epitaxial SrTiO3/DyScO3 films: the ferroelectric soft mode is linearly coupled to a central peak which is silent in the paraelectric phase and it becomes coupled to the polarization below the ferroelectric transition temperature with a progressively increasing bare strength. (en)
Title
  • Ferroelectric phase transition in polycrystalline KTaO3 thin film revealed by terahertz spectroscopy
  • Ferroelectric phase transition in polycrystalline KTaO3 thin film revealed by terahertz spectroscopy (en)
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  • Ferroelectric phase transition in polycrystalline KTaO3 thin film revealed by terahertz spectroscopy
  • Ferroelectric phase transition in polycrystalline KTaO3 thin film revealed by terahertz spectroscopy (en)
skos:notation
  • RIV/68378271:_____/11:00373954!RIV12-AV0-68378271
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  • P(GD202/09/H041), P(IAA100100907), Z(AV0Z10100520)
http://linked.open...iv/cisloPeriodika
  • 5
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  • 199549
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  • RIV/68378271:_____/11:00373954
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  • thin film; terahertz spectroscopy; ferroelectric phase transition (en)
http://linked.open.../riv/klicoveSlovo
http://linked.open...odStatuVydavatele
  • US - Spojené státy americké
http://linked.open...ontrolniKodProRIV
  • [2AD194658E19]
http://linked.open...i/riv/nazevZdroje
  • Applied Physics Letters
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http://linked.open...v/svazekPeriodika
  • 99
http://linked.open...iv/tvurceVysledku
  • Bovtun, Viktor
  • Kosec, M.
  • Kamba, Stanislav
  • Kempa, Martin
  • Kužel, Petr
  • Petzelt, Jan
  • Glinšek, S.
  • Malič, B.
  • Skoromets, Volodymyr
http://linked.open...ain/vavai/riv/wos
  • 000293617300062
http://linked.open...n/vavai/riv/zamer
issn
  • 0003-6951
number of pages
http://bibframe.org/vocab/doi
  • 10.1063/1.3624710
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