About: Effects of high pressure on the structural, magnetic, and transport properties of the itinerant 5 f ferromagnet U2Fe3Ge     Goto   Sponge   NotDistinct   Permalink

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  • Crystal structure, magnetic, and transport properties of the U2Fe3Ge compound have been studied under hydrostatic pressure. U2Fe3Ge crystallizes in the hexagonal crystal structure of the Mg2Cu3Si type, an ordered variant of the MgZn2 Laves structure (C14). The Laves phase has proven highly stable; the crystal structure is maintained up to 27 GPa, the highest applied pressure. X-ray diffraction data revealed that the c direction, where the shortest U-U bonds lie, is softer than the a direction. The bulk modulus B-0 is similar to 100 GPa. U2Fe3Ge is an itinerant ferromagnet with the Curie temperature T-C = 55 K and the spontaneous magnetic moment M-s = 1 mu(B) per formula unit at ambient pressure. The two parameters decrease rapidly under pressure with the rates d(ln M-s)/dp = -0.33 GPa(-1) and d(ln T-C)/dp = -0.27 GPa(-1). The extrapolation of T-C and M-s indicates that the magnetic order will be suppressed between 3 and 4 GPa. Electrical resistivity was found to decrease gradually with increasing pressure. The data in the ferromagnetic state points to the opening of a gap in the magnon spectrum at higher pressures. U2Fe3Ge is relatively more sensitive to pressure than isostructural UNi2.
  • Crystal structure, magnetic, and transport properties of the U2Fe3Ge compound have been studied under hydrostatic pressure. U2Fe3Ge crystallizes in the hexagonal crystal structure of the Mg2Cu3Si type, an ordered variant of the MgZn2 Laves structure (C14). The Laves phase has proven highly stable; the crystal structure is maintained up to 27 GPa, the highest applied pressure. X-ray diffraction data revealed that the c direction, where the shortest U-U bonds lie, is softer than the a direction. The bulk modulus B-0 is similar to 100 GPa. U2Fe3Ge is an itinerant ferromagnet with the Curie temperature T-C = 55 K and the spontaneous magnetic moment M-s = 1 mu(B) per formula unit at ambient pressure. The two parameters decrease rapidly under pressure with the rates d(ln M-s)/dp = -0.33 GPa(-1) and d(ln T-C)/dp = -0.27 GPa(-1). The extrapolation of T-C and M-s indicates that the magnetic order will be suppressed between 3 and 4 GPa. Electrical resistivity was found to decrease gradually with increasing pressure. The data in the ferromagnetic state points to the opening of a gap in the magnon spectrum at higher pressures. U2Fe3Ge is relatively more sensitive to pressure than isostructural UNi2. (en)
Title
  • Effects of high pressure on the structural, magnetic, and transport properties of the itinerant 5 f ferromagnet U2Fe3Ge
  • Effects of high pressure on the structural, magnetic, and transport properties of the itinerant 5 f ferromagnet U2Fe3Ge (en)
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  • Effects of high pressure on the structural, magnetic, and transport properties of the itinerant 5 f ferromagnet U2Fe3Ge
  • Effects of high pressure on the structural, magnetic, and transport properties of the itinerant 5 f ferromagnet U2Fe3Ge (en)
skos:notation
  • RIV/00216208:11320/14:10271614!RIV15-MSM-11320___
http://linked.open...avai/riv/aktivita
http://linked.open...avai/riv/aktivity
  • I, P(GAP204/10/0330), P(GAP204/12/0150), P(LM2011025), S
http://linked.open...iv/cisloPeriodika
  • 5
http://linked.open...vai/riv/dodaniDat
http://linked.open...aciTvurceVysledku
http://linked.open.../riv/druhVysledku
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http://linked.open...dnocenehoVysledku
  • 13731
http://linked.open...ai/riv/idVysledku
  • RIV/00216208:11320/14:10271614
http://linked.open...riv/jazykVysledku
http://linked.open.../riv/klicovaSlova
  • gpa; resistivity; superconductivity; ufe2; uranium-compounds; heavy-fermion compounds (en)
http://linked.open.../riv/klicoveSlovo
http://linked.open...odStatuVydavatele
  • US - Spojené státy americké
http://linked.open...ontrolniKodProRIV
  • [4E7AF1A74432]
http://linked.open...i/riv/nazevZdroje
  • Physical Review B - Condensed Matter and Materials Physics
http://linked.open...in/vavai/riv/obor
http://linked.open...ichTvurcuVysledku
http://linked.open...cetTvurcuVysledku
http://linked.open...vavai/riv/projekt
http://linked.open...UplatneniVysledku
http://linked.open...v/svazekPeriodika
  • 89
http://linked.open...iv/tvurceVysledku
  • Havela, Ladislav
  • Gorbunov, Denis
  • Griveau, J.-C.
  • Goncalves, A. P.
  • Henriques, M. S.
  • Lopes, E. B.
  • Heathman, S.
  • Prchal, Jiří
  • Andreev, A. V.
  • Arnold, Z.
  • Surble, S.
http://linked.open...ain/vavai/riv/wos
  • 000332379900003
issn
  • 1098-0121
number of pages
http://bibframe.org/vocab/doi
  • 10.1103/PhysRevB.89.054407
http://localhost/t...ganizacniJednotka
  • 11320
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