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Description
| - Stavová rovnice Simha-Somcynskeho byla použita k výpočtu volno-objemového parametru h z tlak-objem-teplota (PVT) závislostí osmi polymerů. Predikovaná variance parametru h s teplotou a tlakem byl potvrzen positron anihilační spektroskopií a odpovídající shodabyla nalezena pro h(P=konstantní)=h(T) stejně jako h(T=konstantní)=h(P). Kapilární smyková viskozitní data (v) stejných polymerů pro tři různé teploty a šest tlaků byla vynesena jako funkce log(v) versus 1/h, kdy h bylo vypočítáno pro hodnoty tlaku a teploty experimentálních podmínek viskozitních měření. Dříve nalezená %22master křivka%22 pro silikonové oleje v širokém rozpětí teploty a tlaku byla shledána jako nepoužitelná pro taveniny polymerů. (cs)
- The Simha-Somcynsky (S-S) equation of state (eos) was used to compute the free volume parameter, h, from the pressure-volume-temperature (PVT) dependencies of eight molten polymers. The predicted by eos variation of h with T and P was confirmed by the positron annihilation lifetime spectroscopy; good agreement was found for h(P=constant)=h(T) as well as for h(T=constant)=h(P). Capillary shear viscosity (η) data of the same polymers (measured at three temperatures and six pressures up to 700 bars), were plotted as logη vs 1/h, the latter computed for T and P at which η was measured. In previous works, such a plot for solvents and silicone oils resulted in a %22master curve%22 for the liquid, in a wide range of T and P. However, for molten polymers, no superposition of data onto a %22master curve%22 could be found.
- The Simha-Somcynsky (S-S) equation of state (eos) was used to compute the free volume parameter, h, from the pressure-volume-temperature (PVT) dependencies of eight molten polymers. The predicted by eos variation of h with T and P was confirmed by the positron annihilation lifetime spectroscopy; good agreement was found for h(P=constant)=h(T) as well as for h(T=constant)=h(P). Capillary shear viscosity (η) data of the same polymers (measured at three temperatures and six pressures up to 700 bars), were plotted as logη vs 1/h, the latter computed for T and P at which η was measured. In previous works, such a plot for solvents and silicone oils resulted in a %22master curve%22 for the liquid, in a wide range of T and P. However, for molten polymers, no superposition of data onto a %22master curve%22 could be found. (en)
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Title
| - Free volume dependence of polymer viscosity
- Free volume dependence of polymer viscosity (en)
- Volno-objemová závislost viskozity polymerů (cs)
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skos:prefLabel
| - Free volume dependence of polymer viscosity
- Free volume dependence of polymer viscosity (en)
- Volno-objemová závislost viskozity polymerů (cs)
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skos:notation
| - RIV/70883521:28110/07:63505489!RIV08-AV0-28110___
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http://linked.open.../vavai/riv/strany
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http://linked.open...avai/riv/aktivita
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http://linked.open...avai/riv/aktivity
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http://linked.open...iv/cisloPeriodika
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http://linked.open...vai/riv/dodaniDat
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http://linked.open...aciTvurceVysledku
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http://linked.open.../riv/druhVysledku
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http://linked.open...iv/duvernostUdaju
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http://linked.open...titaPredkladatele
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http://linked.open...dnocenehoVysledku
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http://linked.open...ai/riv/idVysledku
| - RIV/70883521:28110/07:63505489
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http://linked.open...riv/jazykVysledku
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http://linked.open.../riv/klicovaSlova
| - PVT behavior; Equation-of-state; Free volume; Viscosity; Temperature and pressure dependence (en)
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http://linked.open.../riv/klicoveSlovo
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http://linked.open...odStatuVydavatele
| - DE - Spolková republika Německo
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http://linked.open...ontrolniKodProRIV
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http://linked.open...i/riv/nazevZdroje
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http://linked.open...in/vavai/riv/obor
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http://linked.open...ichTvurcuVysledku
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http://linked.open...cetTvurcuVysledku
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http://linked.open...vavai/riv/projekt
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http://linked.open...UplatneniVysledku
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http://linked.open...v/svazekPeriodika
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http://linked.open...iv/tvurceVysledku
| - Sedláček, Tomáš
- Utracki, Leszek
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issn
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number of pages
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http://localhost/t...ganizacniJednotka
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