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Statements

Subject Item
n2:RIV%2F68378271%3A_____%2F14%3A00432547%21RIV15-GA0-68378271
rdf:type
skos:Concept n18:Vysledek
dcterms:description
The electronic configurations of Fe, Co, Ni and Cu adatoms on graphene and graphite have been studied by x-ray magnetic circular dichroism and charge transfer multiplet theory. A delicate interplay between long-range interactions and local chemical bonding is found to influence the adatom equilibrium distance and magnetic moment. The results for Fe and Co are consistent with purely physisorbed species having, however, different 3d-shell occupations on graphene and graphite (dn+1 and dn, respectively). On the other hand, for the late 3d metals Ni and Cu a trend towards chemisorption is found, which strongly quenches the magnetic moment on both substrates. The electronic configurations of Fe, Co, Ni and Cu adatoms on graphene and graphite have been studied by x-ray magnetic circular dichroism and charge transfer multiplet theory. A delicate interplay between long-range interactions and local chemical bonding is found to influence the adatom equilibrium distance and magnetic moment. The results for Fe and Co are consistent with purely physisorbed species having, however, different 3d-shell occupations on graphene and graphite (dn+1 and dn, respectively). On the other hand, for the late 3d metals Ni and Cu a trend towards chemisorption is found, which strongly quenches the magnetic moment on both substrates.
dcterms:title
Single 3d transition metal atoms on multi-layer graphene systems: electronic configurations, bonding mechanisms and role of the substrate Single 3d transition metal atoms on multi-layer graphene systems: electronic configurations, bonding mechanisms and role of the substrate
skos:prefLabel
Single 3d transition metal atoms on multi-layer graphene systems: electronic configurations, bonding mechanisms and role of the substrate Single 3d transition metal atoms on multi-layer graphene systems: electronic configurations, bonding mechanisms and role of the substrate
skos:notation
RIV/68378271:_____/14:00432547!RIV15-GA0-68378271
n3:aktivita
n13:P n13:I
n3:aktivity
I, P(GAP108/11/0853)
n3:cisloPeriodika
Jun
n3:dodaniDat
n14:2015
n3:domaciTvurceVysledku
Honolka, Jan n17:2876663
n3:druhVysledku
n9:J
n3:duvernostUdaju
n15:S
n3:entitaPredkladatele
n5:predkladatel
n3:idSjednocenehoVysledku
45082
n3:idVysledku
RIV/68378271:_____/14:00432547
n3:jazykVysledku
n8:eng
n3:klicovaSlova
graphene; magnetic adsorbates; x-ray absorption spectroscopy; surface magnetism
n3:klicoveSlovo
n4:surface%20magnetism n4:magnetic%20adsorbates n4:x-ray%20absorption%20spectroscopy n4:graphene
n3:kodStatuVydavatele
DE - Spolková republika Německo
n3:kontrolniKodProRIV
[22670A05FAA3]
n3:nazevZdroje
New Journal of Physics
n3:obor
n12:BM
n3:pocetDomacichTvurcuVysledku
2
n3:pocetTvurcuVysledku
11
n3:projekt
n6:GAP108%2F11%2F0853
n3:rokUplatneniVysledku
n14:2014
n3:svazekPeriodika
16
n3:tvurceVysledku
Stepanow, S. Krotzky, S. Rudenko, A. N. Kern, K. Mallet, P. Hiebel, F. Honolka, Jan Veuillen, J.-Y. Brookes, N. B. Sessi, V. Šipr, Ondřej
n3:wos
000339083000001
s:issn
1367-2630
s:numberOfPages
11
n11:doi
10.1088/1367-2630/16/6/062001