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Statements

Subject Item
n2:RIV%2F68378271%3A_____%2F13%3A00397088%21RIV14-GA0-68378271
rdf:type
skos:Concept n10:Vysledek
dcterms:description
Electronic structure calculations combining the local-density approximation with an exact diagonalization of the Anderson impurity model show an intermediate 5f5-5f6-valence ground state and delocalization of the 5f5 multiplet of the Pu atom 5f shell in PuCoIn5, PuCoGa5, and δ-Pu. The 5f local magnetic moment is compensated by a moment formed in the surrounding cloud of conduction electrons. For PuCoGa5 and δ-Pu the compensation is complete, and the Anderson impurity ground state is a singlet. For PuCoIn5 the compensation is partial, and the Pu ground state is magnetic. We suggest that the unconventional d-wave superconductivity is likely mediated by the 5f-state antiferromagnetic fluctuations in PuCoIn5 and by valence fluctuations in PuCoGa5. Electronic structure calculations combining the local-density approximation with an exact diagonalization of the Anderson impurity model show an intermediate 5f5-5f6-valence ground state and delocalization of the 5f5 multiplet of the Pu atom 5f shell in PuCoIn5, PuCoGa5, and δ-Pu. The 5f local magnetic moment is compensated by a moment formed in the surrounding cloud of conduction electrons. For PuCoGa5 and δ-Pu the compensation is complete, and the Anderson impurity ground state is a singlet. For PuCoIn5 the compensation is partial, and the Pu ground state is magnetic. We suggest that the unconventional d-wave superconductivity is likely mediated by the 5f-state antiferromagnetic fluctuations in PuCoIn5 and by valence fluctuations in PuCoGa5.
dcterms:title
Unified character of correlation effects in unconventional Pu-based superconductors and δ-Pu Unified character of correlation effects in unconventional Pu-based superconductors and δ-Pu
skos:prefLabel
Unified character of correlation effects in unconventional Pu-based superconductors and δ-Pu Unified character of correlation effects in unconventional Pu-based superconductors and δ-Pu
skos:notation
RIV/68378271:_____/13:00397088!RIV14-GA0-68378271
n10:predkladatel
n14:ico%3A68378271
n3:aktivita
n4:P n4:I
n3:aktivity
I, P(GAP204/10/0330), P(IAA100100912)
n3:cisloPeriodika
2
n3:dodaniDat
n7:2014
n3:domaciTvurceVysledku
n11:4667026 n11:5138833 n11:4426290
n3:druhVysledku
n18:J
n3:duvernostUdaju
n16:S
n3:entitaPredkladatele
n17:predkladatel
n3:idSjednocenehoVysledku
112599
n3:idVysledku
RIV/68378271:_____/13:00397088
n3:jazykVysledku
n6:eng
n3:klicovaSlova
superconductivity; magnetism; plutonium
n3:klicoveSlovo
n9:superconductivity n9:plutonium n9:magnetism
n3:kodStatuVydavatele
US - Spojené státy americké
n3:kontrolniKodProRIV
[D70D804310EA]
n3:nazevZdroje
Physical Review. B
n3:obor
n19:BM
n3:pocetDomacichTvurcuVysledku
3
n3:pocetTvurcuVysledku
7
n3:projekt
n15:IAA100100912 n15:GAP204%2F10%2F0330
n3:rokUplatneniVysledku
n7:2013
n3:svazekPeriodika
87
n3:tvurceVysledku
Shick, Alexander Oppeneer, P. M. Kolorenč, Jindřich Katsnelson, M. I. Rusz, Ján Lichtenstein, A. I. Caciuffo, R.
n3:wos
000313423900002
s:issn
1098-0121
s:numberOfPages
5
n12:doi
10.1103/PhysRevB.87.020505