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Statements

Subject Item
n2:RIV%2F67985858%3A_____%2F14%3A00436061%21RIV15-AV0-67985858
rdf:type
n8:Vysledek skos:Concept
dcterms:description
A photo microreactor (PMR) of unique parameters was operated in the degradation of 4-chlorophenol with sulfonated zinc phthalocyanine (ZnPcSmix). This sensitizer was chosen as model homogeneous photocatalyst to evaluate operation parameters and efficiency of the PMR. All reactions were carried out in deuterium oxide to maximize the life-time of the generated singlet oxygen species. In parallel same model oxidations were performed in a laboratory batch system using identical optical arrangements. Both systems were optimized and evaluated with help of kinetic models and rationally compared. It was shown the PMR arrangement revealed much higher process efficacy. Construction details and optimized operating parameters of the PMR are provided and discussed in details. A photo microreactor (PMR) of unique parameters was operated in the degradation of 4-chlorophenol with sulfonated zinc phthalocyanine (ZnPcSmix). This sensitizer was chosen as model homogeneous photocatalyst to evaluate operation parameters and efficiency of the PMR. All reactions were carried out in deuterium oxide to maximize the life-time of the generated singlet oxygen species. In parallel same model oxidations were performed in a laboratory batch system using identical optical arrangements. Both systems were optimized and evaluated with help of kinetic models and rationally compared. It was shown the PMR arrangement revealed much higher process efficacy. Construction details and optimized operating parameters of the PMR are provided and discussed in details.
dcterms:title
Microreactor as Efficient Tool for Light Induced Oxidation Reactions Microreactor as Efficient Tool for Light Induced Oxidation Reactions
skos:prefLabel
Microreactor as Efficient Tool for Light Induced Oxidation Reactions Microreactor as Efficient Tool for Light Induced Oxidation Reactions
skos:notation
RIV/67985858:_____/14:00436061!RIV15-AV0-67985858
n3:aktivita
n17:I
n3:aktivity
I
n3:cisloPeriodika
NOV 1
n3:dodaniDat
n16:2015
n3:domaciTvurceVysledku
n4:8824274 n4:5853176 n4:4469380 n4:1946609
n3:druhVysledku
n5:J
n3:duvernostUdaju
n9:S
n3:entitaPredkladatele
n13:predkladatel
n3:idSjednocenehoVysledku
29202
n3:idVysledku
RIV/67985858:_____/14:00436061
n3:jazykVysledku
n14:eng
n3:klicovaSlova
photo microreactor; phthalocyanine; chlorophenol oxidation
n3:klicoveSlovo
n7:photo%20microreactor n7:phthalocyanine n7:chlorophenol%20oxidation
n3:kodStatuVydavatele
NL - Nizozemsko
n3:kontrolniKodProRIV
[B36211F57E63]
n3:nazevZdroje
Chemical Engineering Journal
n3:obor
n15:CI
n3:pocetDomacichTvurcuVysledku
4
n3:pocetTvurcuVysledku
6
n3:rokUplatneniVysledku
n16:2014
n3:svazekPeriodika
255
n3:tvurceVysledku
Klusoň, Petr Křišťál, Jiří Buzek, D. Drhová, Magdalena Hejda, S. Krystyník, Pavel
n3:wos
000341470800023
s:issn
1385-8947
s:numberOfPages
7
n12:doi
10.1016/j.cej.2014.06.052