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Statements

Subject Item
n2:RIV%2F62690094%3A18470%2F13%3A50001687%21RIV14-MSM-18470___
rdf:type
n5:Vysledek skos:Concept
dcterms:description
Absorption and steady state fluorescence spectra of exciton states for ring molecular systems are presented. The peripheral cyclic antenna unit LH4 of the bacterial photosystem from purple bacteria can be modeled by such system. The cumulant-expansion method of Mukamel et al. is used for the calculation of spectral responses of the system with exciton-phonon coupling. Dynamic disorder, interaction with a bath, in Markovian approximation simultaneously with uncorrelated static disorder in transfer integrals are taking into account in our simulations. We compare calculated absorption and steady state fluorescence spectra for LH4 ring obtained within the full Hamiltonian model with our previous results within nearest neighbour approximation model for uncorrelated static disorder in transfer integrals. All calculations were done in software package Mathematica. Absorption and steady state fluorescence spectra of exciton states for ring molecular systems are presented. The peripheral cyclic antenna unit LH4 of the bacterial photosystem from purple bacteria can be modeled by such system. The cumulant-expansion method of Mukamel et al. is used for the calculation of spectral responses of the system with exciton-phonon coupling. Dynamic disorder, interaction with a bath, in Markovian approximation simultaneously with uncorrelated static disorder in transfer integrals are taking into account in our simulations. We compare calculated absorption and steady state fluorescence spectra for LH4 ring obtained within the full Hamiltonian model with our previous results within nearest neighbour approximation model for uncorrelated static disorder in transfer integrals. All calculations were done in software package Mathematica.
dcterms:title
Intermolecular Coupling Fluctuation Effect on Absorption and Emission Spectra for LH4 Ring - Full Hamiltonian Model Intermolecular Coupling Fluctuation Effect on Absorption and Emission Spectra for LH4 Ring - Full Hamiltonian Model
skos:prefLabel
Intermolecular Coupling Fluctuation Effect on Absorption and Emission Spectra for LH4 Ring - Full Hamiltonian Model Intermolecular Coupling Fluctuation Effect on Absorption and Emission Spectra for LH4 Ring - Full Hamiltonian Model
skos:notation
RIV/62690094:18470/13:50001687!RIV14-MSM-18470___
n5:predkladatel
n20:orjk%3A18470
n3:aktivita
n21:S n21:I
n3:aktivity
I, S
n3:dodaniDat
n11:2014
n3:domaciTvurceVysledku
n16:3268721
n3:druhVysledku
n13:D
n3:duvernostUdaju
n17:S
n3:entitaPredkladatele
n7:predkladatel
n3:idSjednocenehoVysledku
80785
n3:idVysledku
RIV/62690094:18470/13:50001687
n3:jazykVysledku
n4:eng
n3:klicovaSlova
Mathematica; localization; exciton states; static and dynamic disorder; absorption and fluorescence spectrum; LH4
n3:klicoveSlovo
n6:absorption%20and%20fluorescence%20spectrum n6:static%20and%20dynamic%20disorder n6:localization n6:exciton%20states n6:Mathematica n6:LH4
n3:kontrolniKodProRIV
[C6BD72194C12]
n3:mistoKonaniAkce
Budapešť, Maďarsko
n3:mistoVydani
Athens
n3:nazevZdroje
Applied mathematics (AMATH '13) : proceedings of the 18th WSEAS international conference
n3:obor
n19:BA
n3:pocetDomacichTvurcuVysledku
1
n3:pocetTvurcuVysledku
2
n3:rokUplatneniVysledku
n11:2013
n3:tvurceVysledku
Heřman, Pavel Zapletal, David
n3:typAkce
n10:WRD
n3:zahajeniAkce
2013-12-10+01:00
s:issn
2227-4588
s:numberOfPages
6
n15:hasPublisher
World scientific and engineering academy and society
n18:isbn
978-960-474-351-3
n9:organizacniJednotka
18470