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Statements

Subject Item
n2:RIV%2F61989592%3A15310%2F14%3A33152591%21RIV15-MSM-15310___
rdf:type
n15:Vysledek skos:Concept
rdfs:seeAlso
http://www.sciencedirect.com/science/article/pii/S1385894714007761
dcterms:description
A novel graphitic carbon nitride (GCN) material has been synthesized through a low-temperature solvolysis of sodium cyanide in formamide. The structure and morphology of the so-obtained GCN solid were studied by X-ray diffraction (XRD), transmission electron microscopy (TEM), Raman/Infrared (IR) spectroscopy and thermal gravimetric analysis (TGA). GCN is characterized by a compacted layered structure bearing a high content of pendant amine groups (1.4 mmol g1). Electron Paramagnetic Resonance spectroscopy reveals that the pendant amine groups are readily accessible by extrinsic metal cations. Moreover, GCN has a considerable electron-donating capacity to adsorbed electron accepting ions such as Cu2+.GCN shows an appreciable As(III) uptake capacity of 39.7 mg g1. Based on theoretical Surface Complexation Model we provide a consistent interfacial/structural picture that describes quantitatively observed phenomena. A novel graphitic carbon nitride (GCN) material has been synthesized through a low-temperature solvolysis of sodium cyanide in formamide. The structure and morphology of the so-obtained GCN solid were studied by X-ray diffraction (XRD), transmission electron microscopy (TEM), Raman/Infrared (IR) spectroscopy and thermal gravimetric analysis (TGA). GCN is characterized by a compacted layered structure bearing a high content of pendant amine groups (1.4 mmol g1). Electron Paramagnetic Resonance spectroscopy reveals that the pendant amine groups are readily accessible by extrinsic metal cations. Moreover, GCN has a considerable electron-donating capacity to adsorbed electron accepting ions such as Cu2+.GCN shows an appreciable As(III) uptake capacity of 39.7 mg g1. Based on theoretical Surface Complexation Model we provide a consistent interfacial/structural picture that describes quantitatively observed phenomena.
dcterms:title
Arsenite remediation by an amine-rich graphitic carbon nitride synthesized by a novel low-temperature method Arsenite remediation by an amine-rich graphitic carbon nitride synthesized by a novel low-temperature method
skos:prefLabel
Arsenite remediation by an amine-rich graphitic carbon nitride synthesized by a novel low-temperature method Arsenite remediation by an amine-rich graphitic carbon nitride synthesized by a novel low-temperature method
skos:notation
RIV/61989592:15310/14:33152591!RIV15-MSM-15310___
n3:aktivita
n16:P
n3:aktivity
P(ED2.1.00/03.0058), P(EE2.3.20.0155)
n3:cisloPeriodika
NOV
n3:dodaniDat
n4:2015
n3:domaciTvurceVysledku
n13:9251189
n3:druhVysledku
n11:J
n3:duvernostUdaju
n18:S
n3:entitaPredkladatele
n17:predkladatel
n3:idSjednocenehoVysledku
4121
n3:idVysledku
RIV/61989592:15310/14:33152591
n3:jazykVysledku
n7:eng
n3:klicovaSlova
FITEQL,EPR; Surface Complexation Modeling; Arsenite remediation; Low-temperature solvolysis; Carbon nitride
n3:klicoveSlovo
n10:Carbon%20nitride n10:EPR n10:FITEQL n10:Arsenite%20remediation n10:Low-temperature%20solvolysis n10:Surface%20Complexation%20Modeling
n3:kodStatuVydavatele
NL - Nizozemsko
n3:kontrolniKodProRIV
[AA4862598507]
n3:nazevZdroje
Chemical Engineering Journal
n3:obor
n14:CA
n3:pocetDomacichTvurcuVysledku
1
n3:pocetTvurcuVysledku
8
n3:projekt
n6:ED2.1.00%2F03.0058 n6:EE2.3.20.0155
n3:rokUplatneniVysledku
n4:2014
n3:svazekPeriodika
256
n3:tvurceVysledku
Daikopoulos, Chris Steriotis, T A Georgiou, Yiannis Baikousi, Maria Bourlinos, Athanasios Zbořil, Radek Deligiannakis, Yiannis G Karakassides, Michael A.
n3:wos
000341558400036
s:issn
1385-8947
s:numberOfPages
9
n20:doi
10.1016/j.cej.2014.06.045
n19:organizacniJednotka
15310