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Statements

Subject Item
n2:RIV%2F61389013%3A_____%2F14%3A00435100%21RIV15-GA0-61389013
rdf:type
n7:Vysledek skos:Concept
dcterms:description
This study is focused on thermoresponsive glycogen-graft-poly(2-alkyl-2-oxazolines), a new group of nanostructured hybrid dendrimeric stimuli-responsive polymers connecting the body’s own biodegradable polysaccharidic dendrimer glycogen with the widely tuneable thermoresponsive behavior of polypeptide-analogic poly(2-alkyl-2-oxazolines), which are known to be biocompatible. Glycogen-graft-poly(2-alkyl-2-oxazolines) were prepared by a simple one-pot two-step procedure involving cationic ring-opening polymerization of 2-alkyl-2-oxazolines followed by termination of the living cationic ends with sodium glycogenate. As confirmed by light and X-ray scattering, as well as cryo-transmission electron microscopy, the grafted dendrimer structure allows easy adjustment of the cloud point temperature, the concentration dependence and nanostructure of the self-assembled phase separated polymer by crosstalk during graft composition, the graft length and the grafting density, in a very wide range. This study is focused on thermoresponsive glycogen-graft-poly(2-alkyl-2-oxazolines), a new group of nanostructured hybrid dendrimeric stimuli-responsive polymers connecting the body’s own biodegradable polysaccharidic dendrimer glycogen with the widely tuneable thermoresponsive behavior of polypeptide-analogic poly(2-alkyl-2-oxazolines), which are known to be biocompatible. Glycogen-graft-poly(2-alkyl-2-oxazolines) were prepared by a simple one-pot two-step procedure involving cationic ring-opening polymerization of 2-alkyl-2-oxazolines followed by termination of the living cationic ends with sodium glycogenate. As confirmed by light and X-ray scattering, as well as cryo-transmission electron microscopy, the grafted dendrimer structure allows easy adjustment of the cloud point temperature, the concentration dependence and nanostructure of the self-assembled phase separated polymer by crosstalk during graft composition, the graft length and the grafting density, in a very wide range.
dcterms:title
Glycogen-graft-poly(2-alkyl-2-oxazolines) - the new versatile biopolymer-based thermoresponsive macromolecular toolbox Glycogen-graft-poly(2-alkyl-2-oxazolines) - the new versatile biopolymer-based thermoresponsive macromolecular toolbox
skos:prefLabel
Glycogen-graft-poly(2-alkyl-2-oxazolines) - the new versatile biopolymer-based thermoresponsive macromolecular toolbox Glycogen-graft-poly(2-alkyl-2-oxazolines) - the new versatile biopolymer-based thermoresponsive macromolecular toolbox
skos:notation
RIV/61389013:_____/14:00435100!RIV15-GA0-61389013
n3:aktivita
n5:P n5:I
n3:aktivity
I, P(GA13-08336S), P(LH14079)
n3:cisloPeriodika
106
n3:dodaniDat
n10:2015
n3:domaciTvurceVysledku
n4:8685509 Bogomolova, Anna n4:2540568 n4:1474545 n4:9218424 Matushkin, Nikolai Filippov, Sergey n4:2069652
n3:druhVysledku
n17:J
n3:duvernostUdaju
n15:S
n3:entitaPredkladatele
n14:predkladatel
n3:idSjednocenehoVysledku
18452
n3:idVysledku
RIV/61389013:_____/14:00435100
n3:jazykVysledku
n11:eng
n3:klicovaSlova
glycogen; poly(2-alkyl-2-oxazoline); hybrid copolymer
n3:klicoveSlovo
n12:glycogen n12:poly%282-alkyl-2-oxazoline%29 n12:hybrid%20copolymer
n3:kodStatuVydavatele
GB - Spojené království Velké Británie a Severního Irska
n3:kontrolniKodProRIV
[89D22265E0FA]
n3:nazevZdroje
RSC Advances
n3:obor
n16:CD
n3:pocetDomacichTvurcuVysledku
8
n3:pocetTvurcuVysledku
9
n3:projekt
n9:GA13-08336S n9:LH14079
n3:rokUplatneniVysledku
n10:2014
n3:svazekPeriodika
4
n3:tvurceVysledku
Turner, S. Pospíšilová, Aneta Sedláček, Ondřej Matushkin, Nikolai Filippov, Sergey Hrubý, Martin Bogomolova, Anna Štěpánek, Petr Černochová, Zulfiya
n3:wos
000345656600045
s:issn
2046-2069
s:numberOfPages
9
n18:doi
10.1039/C4RA10315G