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Statements

Subject Item
n2:RIV%2F61388963%3A_____%2F14%3A00439691%21RIV15-GA0-61388963
rdf:type
n5:Vysledek skos:Concept
dcterms:description
The vibrational states of atomic and molecular particles adsorbed on long linear nanographenes are described using reliable theoretical potentials and appropriate vibrational (lateral) Hamiltonians. Although they rigorously obey the Bloch theorem only for infinite nanographenes, the energy patterns of the probed states closely resemble the usual Bloch bands and gaps. In addition, for any finite nanographene, these patterns are enriched by the presence of “solitary energy levels and the “resonance structure of the bands. While typical band states are profoundly delocalised due to a fast tunneling of the adsorbed particle, the “solitary and “resonance states exhibit strong localisation, similar to the behaviour of the states of the Wannier-Stark ladders in optical and semiconductor superlattices. The vibrational states of atomic and molecular particles adsorbed on long linear nanographenes are described using reliable theoretical potentials and appropriate vibrational (lateral) Hamiltonians. Although they rigorously obey the Bloch theorem only for infinite nanographenes, the energy patterns of the probed states closely resemble the usual Bloch bands and gaps. In addition, for any finite nanographene, these patterns are enriched by the presence of “solitary energy levels and the “resonance structure of the bands. While typical band states are profoundly delocalised due to a fast tunneling of the adsorbed particle, the “solitary and “resonance states exhibit strong localisation, similar to the behaviour of the states of the Wannier-Stark ladders in optical and semiconductor superlattices.
dcterms:title
Localised quantum states of atomic and molecular particles physisorbed on carbon-based nanoparticles Localised quantum states of atomic and molecular particles physisorbed on carbon-based nanoparticles
skos:prefLabel
Localised quantum states of atomic and molecular particles physisorbed on carbon-based nanoparticles Localised quantum states of atomic and molecular particles physisorbed on carbon-based nanoparticles
skos:notation
RIV/61388963:_____/14:00439691!RIV15-GA0-61388963
n3:aktivita
n11:P n11:I
n3:aktivity
I, P(GAP205/11/0571), P(GAP208/10/0725), P(GAP208/11/0436)
n3:cisloPeriodika
11
n3:dodaniDat
n15:2015
n3:domaciTvurceVysledku
n4:7734700 n4:4095065 n4:5865875
n3:druhVysledku
n12:J
n3:duvernostUdaju
n7:S
n3:entitaPredkladatele
n18:predkladatel
n3:idSjednocenehoVysledku
26472
n3:idVysledku
RIV/61388963:_____/14:00439691
n3:jazykVysledku
n13:eng
n3:klicovaSlova
periodic structure; carbon nanostructures; graphene; quantum mechanics; physisorbed
n3:klicoveSlovo
n9:physisorbed n9:graphene n9:periodic%20structure n9:carbon%20nanostructures n9:quantum%20mechanics
n3:kodStatuVydavatele
US - Spojené státy americké
n3:kontrolniKodProRIV
[0440900CB196]
n3:nazevZdroje
Journal of Chemical Physics
n3:obor
n17:BG
n3:pocetDomacichTvurcuVysledku
3
n3:pocetTvurcuVysledku
4
n3:projekt
n6:GAP208%2F10%2F0725 n6:GAP208%2F11%2F0436 n6:GAP205%2F11%2F0571
n3:rokUplatneniVysledku
n15:2014
n3:svazekPeriodika
141
n3:tvurceVysledku
Trachta, Michal Kaprálová-Žďánská, Petra Ruth Špirko, Vladimír Bludský, Ota
n3:wos
000342843200029
s:issn
0021-9606
s:numberOfPages
10
n16:doi
10.1063/1.4894412