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Statements

Subject Item
n2:RIV%2F61388955%3A_____%2F13%3A00420720%21RIV14-MPO-61388955
rdf:type
n12:Vysledek skos:Concept
dcterms:description
High-silica zeolites with crystalline aluminosilicate frame- works balance the charge of strongly acidic protons during the processing of oil, in petrochemistry, and increasingly in numerous organic syntheses. The transformation of hydro- carbons is controlled by the concentration and strength of the acid sites and the dimensions and architecture of the inner pores. Zeolite micropores, which have a diameter similar to organic molecules, govern the shape selectivity of the reaction in the inner space, but also result in slow transport of reactants and products, thus limiting the reaction rate. [1] Several approaches have been developed to enhance the mass transport by using zeolite nanosheets and nanocrystals, [2–4] or zeolites that contain both micro- and mesopores. The latter hierarchical zeolites were prepared by confined crystal growth, [5,6] by using polymers as mesoporogens, [7] or through post-synthesis desilication or dealumination processes. High-silica zeolites with crystalline aluminosilicate frame- works balance the charge of strongly acidic protons during the processing of oil, in petrochemistry, and increasingly in numerous organic syntheses. The transformation of hydro- carbons is controlled by the concentration and strength of the acid sites and the dimensions and architecture of the inner pores. Zeolite micropores, which have a diameter similar to organic molecules, govern the shape selectivity of the reaction in the inner space, but also result in slow transport of reactants and products, thus limiting the reaction rate. [1] Several approaches have been developed to enhance the mass transport by using zeolite nanosheets and nanocrystals, [2–4] or zeolites that contain both micro- and mesopores. The latter hierarchical zeolites were prepared by confined crystal growth, [5,6] by using polymers as mesoporogens, [7] or through post-synthesis desilication or dealumination processes.
dcterms:title
Enhancement of Activity and Selectivity in Acid-Catalyzed Reactions by Dealuminated Hierarchical Zeolites Enhancement of Activity and Selectivity in Acid-Catalyzed Reactions by Dealuminated Hierarchical Zeolites
skos:prefLabel
Enhancement of Activity and Selectivity in Acid-Catalyzed Reactions by Dealuminated Hierarchical Zeolites Enhancement of Activity and Selectivity in Acid-Catalyzed Reactions by Dealuminated Hierarchical Zeolites
skos:notation
RIV/61388955:_____/13:00420720!RIV14-MPO-61388955
n12:predkladatel
n18:ico%3A61388955
n3:aktivita
n5:I n5:P
n3:aktivity
I, P(FR-TI3/316), P(GAP106/11/0624)
n3:cisloPeriodika
7
n3:dodaniDat
n10:2014
n3:domaciTvurceVysledku
n11:5120500 n11:9628983 n11:9817034 n11:8844380 n11:3023338 n11:7579543
n3:druhVysledku
n4:J
n3:duvernostUdaju
n14:S
n3:entitaPredkladatele
n8:predkladatel
n3:idSjednocenehoVysledku
72938
n3:idVysledku
RIV/61388955:_____/13:00420720
n3:jazykVysledku
n19:eng
n3:klicovaSlova
alkylation; cracking; dealumination
n3:klicoveSlovo
n7:alkylation n7:cracking n7:dealumination
n3:kodStatuVydavatele
DE - Spolková republika Německo
n3:kontrolniKodProRIV
[0C4178341456]
n3:nazevZdroje
Angewandte Chemie. International Edition in English
n3:obor
n9:CF
n3:pocetDomacichTvurcuVysledku
6
n3:pocetTvurcuVysledku
8
n3:projekt
n16:FR-TI3%2F316 n16:GAP106%2F11%2F0624
n3:rokUplatneniVysledku
n10:2013
n3:svazekPeriodika
52
n3:tvurceVysledku
Sazama, Petr Dědeček, Jiří Sobalík, Zdeněk Parvulescu, V. I. Bastl, Zdeněk Jirglová, Hana Rathouský, Jiří Jakubec, Ivo
n3:wos
000314654000028
s:issn
1433-7851
s:numberOfPages
4
n13:doi
10.1002/anie.201206557