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Statements

Subject Item
n2:RIV%2F61388955%3A_____%2F11%3A00349494%21RIV12-GA0-61388955
rdf:type
n4:Vysledek skos:Concept
dcterms:description
We review our recent results on the photodissociation of hydrogen bonded clusters. They are generated in supersonic expansion and subsequently photolyzed. Hydrogen atoms leaving the clusters are detected and the kinetic energy distributions (KEDs) of these outgoing fragments are determined. In the KED spectra, we distinguish three regimes with an increasing kinetic energy: those products which are slowed down by the cluster cage, those which leave it unperturbed and those which gain energy in processes following primary photodissociation. We have analyzed the shapes of the kinetic energy spectra and identified important reaction channels. Our experiments are accompanied and interpreted with theoretical calculations which are based on state-of the-art ab initio methods, We review our recent results on the photodissociation of hydrogen bonded clusters. They are generated in supersonic expansion and subsequently photolyzed. Hydrogen atoms leaving the clusters are detected and the kinetic energy distributions (KEDs) of these outgoing fragments are determined. In the KED spectra, we distinguish three regimes with an increasing kinetic energy: those products which are slowed down by the cluster cage, those which leave it unperturbed and those which gain energy in processes following primary photodissociation. We have analyzed the shapes of the kinetic energy spectra and identified important reaction channels. Our experiments are accompanied and interpreted with theoretical calculations which are based on state-of the-art ab initio methods,
dcterms:title
Photodissociation of Molecules in Hydrogen Bonded Clusters Probing the Excited State Photodissociation of Molecules in Hydrogen Bonded Clusters Probing the Excited State
skos:prefLabel
Photodissociation of Molecules in Hydrogen Bonded Clusters Probing the Excited State Photodissociation of Molecules in Hydrogen Bonded Clusters Probing the Excited State
skos:notation
RIV/61388955:_____/11:00349494!RIV12-GA0-61388955
n4:predkladatel
n5:ico%3A61388955
n3:aktivita
n16:Z n16:P
n3:aktivity
P(GA203/09/0422), P(KAN400400651), Z(AV0Z40400503)
n3:dodaniDat
n11:2012
n3:domaciTvurceVysledku
n20:1866877
n3:druhVysledku
n9:C
n3:duvernostUdaju
n17:S
n3:entitaPredkladatele
n12:predkladatel
n3:idSjednocenehoVysledku
220243
n3:idVysledku
RIV/61388955:_____/11:00349494
n3:jazykVysledku
n19:eng
n3:klicovaSlova
photodissociation; hydrogen bonded clusters; pure and doped water clusters
n3:klicoveSlovo
n7:pure%20and%20doped%20water%20clusters n7:photodissociation n7:hydrogen%20bonded%20clusters
n3:kontrolniKodProRIV
[6F0E1D34342C]
n3:mistoVydani
Chichester
n3:nazevZdroje
Hydrogen Bonding and Transfer in the Excited State
n3:obor
n18:CF
n3:pocetDomacichTvurcuVysledku
1
n3:pocetStranKnihy
907
n3:pocetTvurcuVysledku
3
n3:projekt
n15:KAN400400651 n15:GA203%2F09%2F0422
n3:rokUplatneniVysledku
n11:2011
n3:tvurceVysledku
Slavíček, P. Buck, U. Fárník, Michal
n3:zamer
n6:AV0Z40400503
s:numberOfPages
27
n21:hasPublisher
John Wiley & Sons Ltd
n14:isbn
978-0-470-66677-7