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Statements

Subject Item
n2:RIV%2F61388955%3A_____%2F05%3A00000604%21RIV06-AV0-61388955
rdf:type
skos:Concept n13:Vysledek
dcterms:description
Phase-pure TiO2(B) with microfibrous morphology was prepared via a newly developed method from amorphous TiO2. Cyclic voltammetry evidences that Li-insertion into TiO2(B) is governed by a pseudocapacitive faradaic process, whose rate is not limited by solid-state diffusion of Li+ in a broad interval of scan rates. This unusual behavior was discussed in terms of the crystal structure of the TiO2(B) host, having freely accessible parallel channels for Li+-transport perpendicular to the (010) face. The characteristic Li-insertion electrochemistry of TiO2(B) allows re-interpretation of several previous reports, which did not consider explicitly this relation or the presence of TiO2(B) in various TiO2 materials of different origin. Phase-pure TiO2(B) with microfibrous morphology was prepared via a newly developed method from amorphous TiO2. Cyclic voltammetry evidences that Li-insertion into TiO2(B) is governed by a pseudocapacitive faradaic process, whose rate is not limited by solid-state diffusion of Li+ in a broad interval of scan rates. This unusual behavior was discussed in terms of the crystal structure of the TiO2(B) host, having freely accessible parallel channels for Li+-transport perpendicular to the (010) face. The characteristic Li-insertion electrochemistry of TiO2(B) allows re-interpretation of several previous reports, which did not consider explicitly this relation or the presence of TiO2(B) in various TiO2 materials of different origin. Byl vyvinut nový syntézní postup pro přípravu fázově čistého TiO2(B) s vláknitou morfologií. Cyklická voltametrie ukázala, že inserce lithia do uvedeného materiálu probíhá jako pseudokapacitní faradaický process, jehož rychlost není limitována difúzí Li dovnitř tuhé fáze pro široký interval rychlostí skenu.
dcterms:title
Pseudokapacitní akumulace lithia v TiO2(B) Pseudocapacitive lithium storage in TiO2(B) Pseudocapacitive lithium storage in TiO2(B)
skos:prefLabel
Pseudocapacitive lithium storage in TiO2(B) Pseudocapacitive lithium storage in TiO2(B) Pseudokapacitní akumulace lithia v TiO2(B)
skos:notation
RIV/61388955:_____/05:00000604!RIV06-AV0-61388955
n3:strany
1248;1255
n3:aktivita
n14:P n14:Z
n3:aktivity
P(1M0577), P(1P04OCD14.10), P(GA203/03/0824), P(GD203/03/H140), Z(AV0Z40400503)
n3:cisloPeriodika
5
n3:dodaniDat
n8:2006
n3:domaciTvurceVysledku
n6:5808111 n6:9704418 n6:1157744
n3:druhVysledku
n12:J
n3:duvernostUdaju
n17:S
n3:entitaPredkladatele
n4:predkladatel
n3:idSjednocenehoVysledku
539582
n3:idVysledku
RIV/61388955:_____/05:00000604
n3:jazykVysledku
n18:eng
n3:klicovaSlova
protonic layered tetratitanate; anatase TiO2; nanocrystalline anotase; transformation
n3:klicoveSlovo
n7:protonic%20layered%20tetratitanate n7:anatase%20TiO2 n7:transformation n7:nanocrystalline%20anotase
n3:kodStatuVydavatele
US - Spojené státy americké
n3:kontrolniKodProRIV
[34C7669FF802]
n3:nazevZdroje
Chemistry of Materials
n3:obor
n15:CG
n3:pocetDomacichTvurcuVysledku
3
n3:pocetTvurcuVysledku
5
n3:projekt
n10:GA203%2F03%2F0824 n10:GD203%2F03%2FH140 n10:1P04OCD14.10 n10:1M0577
n3:rokUplatneniVysledku
n8:2005
n3:svazekPeriodika
17
n3:tvurceVysledku
Grätzel, M. Kalbáč, Martin Zukalová, Markéta Exnar, I. Kavan, Ladislav
n3:zamer
n11:AV0Z40400503
s:issn
0897-4756
s:numberOfPages
8