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Statements

Subject Item
n2:RIV%2F60461373%3A22340%2F14%3A43898189%21RIV15-GA0-22340___
rdf:type
n7:Vysledek skos:Concept
dcterms:description
Paper presents stability analysis of the reaction network corresponding to the mechanism of simultaneous oxidation of carbon monoxide CO, unburned hydrocarbons represented by acetylene C2H2 and reduction of nitrogen oxides NOx , taking place in the three-way catalytic converter used in cars to remove noxious components from exhaust gases. We use stoichiometric network analysis as a method for decomposing the entire mechanism into irreducible subnetworks (extreme currents) and examining stability of corresponding steady states. This methods allows for indication of those subnetworks, which may within a range of control parameters display instabilities leading to oscillations. Within those subnetworks the major positive and negative feedbacks are used to explain the oscillatory dynamics in chemical terms. Paper presents stability analysis of the reaction network corresponding to the mechanism of simultaneous oxidation of carbon monoxide CO, unburned hydrocarbons represented by acetylene C2H2 and reduction of nitrogen oxides NOx , taking place in the three-way catalytic converter used in cars to remove noxious components from exhaust gases. We use stoichiometric network analysis as a method for decomposing the entire mechanism into irreducible subnetworks (extreme currents) and examining stability of corresponding steady states. This methods allows for indication of those subnetworks, which may within a range of control parameters display instabilities leading to oscillations. Within those subnetworks the major positive and negative feedbacks are used to explain the oscillatory dynamics in chemical terms.
dcterms:title
Stoichiometric networks and dynamical instabilities in a model of three way catalytic converter Stoichiometric networks and dynamical instabilities in a model of three way catalytic converter
skos:prefLabel
Stoichiometric networks and dynamical instabilities in a model of three way catalytic converter Stoichiometric networks and dynamical instabilities in a model of three way catalytic converter
skos:notation
RIV/60461373:22340/14:43898189!RIV15-GA0-22340___
n4:aktivita
n17:P
n4:aktivity
P(GA203/09/2091)
n4:dodaniDat
n12:2015
n4:domaciTvurceVysledku
n13:4246039 n13:2329689 n13:4462610
n4:druhVysledku
n6:D
n4:duvernostUdaju
n14:S
n4:entitaPredkladatele
n21:predkladatel
n4:idSjednocenehoVysledku
47567
n4:idVysledku
RIV/60461373:22340/14:43898189
n4:jazykVysledku
n18:eng
n4:klicovaSlova
stoichiometric network analysis; kinetic autocatalysis; catalytic converter
n4:klicoveSlovo
n8:stoichiometric%20network%20analysis n8:kinetic%20autocatalysis n8:catalytic%20converter
n4:kontrolniKodProRIV
[192948F42AF2]
n4:mistoKonaniAkce
Bělehrad
n4:mistoVydani
Bělehrad
n4:nazevZdroje
Physical Chemistry 2014 (Proceedings)
n4:obor
n9:CI
n4:pocetDomacichTvurcuVysledku
3
n4:pocetTvurcuVysledku
3
n4:projekt
n15:GA203%2F09%2F2091
n4:rokUplatneniVysledku
n12:2014
n4:tvurceVysledku
Kohout, Martin Hadač, Otto Schreiber, Igor
n4:typAkce
n19:WRD
n4:zahajeniAkce
2014-09-22+02:00
s:numberOfPages
8
n3:hasPublisher
Society of Physical Chemists of Serbia
n16:isbn
978-86-82475-30-9
n5:organizacniJednotka
22340