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Statements

Subject Item
n2:RIV%2F60461373%3A22340%2F11%3A43891834%21RIV12-MSM-22340___
rdf:type
skos:Concept n15:Vysledek
dcterms:description
The mechanism of photochemistry in the mesopause region entails a chemical oscillator forced by solar short-wave radiation. A model with periodic forcing between day and night conditions produces nonlinear dynamics including period-doubling bifurcations and chaos. The photochemical mechanism represents a network involving positive and negative feedbacks that can be examined by methods of stoichiometric network analysis. We use these methods to decompose the network into irreducible subnetworks and then apply linear stability analysis to find all possible sources of oscillatory instabilities in the mesopause chemistry. These oscillators are classified according to topological features in their reaction networks and phase shifts of oscillating species. We subsequently compare phase shifts indicated by the network analysis with those from direct simulations to identify a specific subnetwork in the mechanism underlying the complex oscillatory dynamics observed in earlier simulations. The mechanism of photochemistry in the mesopause region entails a chemical oscillator forced by solar short-wave radiation. A model with periodic forcing between day and night conditions produces nonlinear dynamics including period-doubling bifurcations and chaos. The photochemical mechanism represents a network involving positive and negative feedbacks that can be examined by methods of stoichiometric network analysis. We use these methods to decompose the network into irreducible subnetworks and then apply linear stability analysis to find all possible sources of oscillatory instabilities in the mesopause chemistry. These oscillators are classified according to topological features in their reaction networks and phase shifts of oscillating species. We subsequently compare phase shifts indicated by the network analysis with those from direct simulations to identify a specific subnetwork in the mechanism underlying the complex oscillatory dynamics observed in earlier simulations.
dcterms:title
Stoichiometric network analysis of the photochemical processes in the mesopause region Stoichiometric network analysis of the photochemical processes in the mesopause region
skos:prefLabel
Stoichiometric network analysis of the photochemical processes in the mesopause region Stoichiometric network analysis of the photochemical processes in the mesopause region
skos:notation
RIV/60461373:22340/11:43891834!RIV12-MSM-22340___
n15:predkladatel
n18:orjk%3A22340
n3:aktivita
n5:P n5:Z n5:S
n3:aktivity
P(GA203/09/2091), P(GD104/08/H055), S, Z(MSM6046137306)
n3:cisloPeriodika
4
n3:dodaniDat
n16:2012
n3:domaciTvurceVysledku
n6:2329689 n6:4462610
n3:druhVysledku
n10:J
n3:duvernostUdaju
n20:S
n3:entitaPredkladatele
n21:predkladatel
n3:idSjednocenehoVysledku
232439
n3:idVysledku
RIV/60461373:22340/11:43891834
n3:jazykVysledku
n13:eng
n3:klicovaSlova
flux; model; mesosphere; photolysis; water; system; bahavior; irradiance; solar; Reaction mechanisms
n3:klicoveSlovo
n4:water n4:mesosphere n4:irradiance n4:model n4:bahavior n4:solar n4:photolysis n4:flux n4:system n4:Reaction%20mechanisms
n3:kodStatuVydavatele
GB - Spojené království Velké Británie a Severního Irska
n3:kontrolniKodProRIV
[957F908AAEF3]
n3:nazevZdroje
Physical Chemistry Chemical Physics
n3:obor
n12:CI
n3:pocetDomacichTvurcuVysledku
2
n3:pocetTvurcuVysledku
2
n3:projekt
n7:GD104%2F08%2FH055 n7:GA203%2F09%2F2091
n3:rokUplatneniVysledku
n16:2011
n3:svazekPeriodika
13
n3:tvurceVysledku
Hadač, Otto Schreiber, Igor
n3:wos
000286056400008
n3:zamer
n17:MSM6046137306
s:issn
1463-9076
s:numberOfPages
9
n19:doi
10.1039/c0cp01267j
n11:organizacniJednotka
22340