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Statements

Subject Item
n2:RIV%2F00216305%3A26620%2F14%3APU112493%21RIV15-MSM-26620___
rdf:type
skos:Concept n14:Vysledek
dcterms:description
Networks combining physical and covalent chemical cross-links can exhibit a large amount of dissipated inelastic energy along with high stretchability during deformation. We present our analysis of the influence of the extent of covalent cross-linking on the inelasticity of hydrogels. Four model networks, which are similar in structure but strongly differ in elasticity, have been studied. The aim was the identification of a key structural factor responsible for observing a hysteresis or an elastic deformation. In the employed molecular dynamics study this factor is derived from the underlying structure of each particular hydrogel network. Several structural characteristics have been investigated like the extent of damage to the network, chains sliding, and the specific properties of load-bearing chains. By means of such a key factor, one can predict the deformation behavior (hysteresis or elasticity) of some material, provided a precise description of its structure exists and it resembles any of the f Networks combining physical and covalent chemical cross-links can exhibit a large amount of dissipated inelastic energy along with high stretchability during deformation. We present our analysis of the influence of the extent of covalent cross-linking on the inelasticity of hydrogels. Four model networks, which are similar in structure but strongly differ in elasticity, have been studied. The aim was the identification of a key structural factor responsible for observing a hysteresis or an elastic deformation. In the employed molecular dynamics study this factor is derived from the underlying structure of each particular hydrogel network. Several structural characteristics have been investigated like the extent of damage to the network, chains sliding, and the specific properties of load-bearing chains. By means of such a key factor, one can predict the deformation behavior (hysteresis or elasticity) of some material, provided a precise description of its structure exists and it resembles any of the f
dcterms:title
Mechanical response of hybrid cross-linked networks to uniaxial deformation: A molecular dynamics model Mechanical response of hybrid cross-linked networks to uniaxial deformation: A molecular dynamics model
skos:prefLabel
Mechanical response of hybrid cross-linked networks to uniaxial deformation: A molecular dynamics model Mechanical response of hybrid cross-linked networks to uniaxial deformation: A molecular dynamics model
skos:notation
RIV/00216305:26620/14:PU112493!RIV15-MSM-26620___
n3:aktivita
n17:P
n3:aktivity
P(ED1.1.00/02.0068)
n3:cisloPeriodika
24
n3:dodaniDat
n7:2015
n3:domaciTvurceVysledku
n5:9608486 n5:1397605
n3:druhVysledku
n13:J
n3:duvernostUdaju
n19:S
n3:entitaPredkladatele
n4:predkladatel
n3:idSjednocenehoVysledku
28086
n3:idVysledku
RIV/00216305:26620/14:PU112493
n3:jazykVysledku
n10:eng
n3:klicovaSlova
molecular dynamics, hydrogel, tensile deformation
n3:klicoveSlovo
n8:tensile%20deformation n8:hydrogel n8:molecular%20dynamics
n3:kodStatuVydavatele
US - Spojené státy americké
n3:kontrolniKodProRIV
[7AB054E63294]
n3:nazevZdroje
MACROMOLECULES
n3:obor
n18:CD
n3:pocetDomacichTvurcuVysledku
2
n3:pocetTvurcuVysledku
4
n3:projekt
n9:ED1.1.00%2F02.0068
n3:rokUplatneniVysledku
n7:2014
n3:svazekPeriodika
47
n3:tvurceVysledku
Vilgis, Thomas Milchev, Andrey Jančář, Josef Žídek, Jan
s:issn
0024-9297
s:numberOfPages
13
n16:doi
10.1021/ma501504z
n15:organizacniJednotka
26620