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Statements

Subject Item
n2:RIV%2F00216275%3A25310%2F14%3A39898158%21RIV15-GA0-25310___
rdf:type
n12:Vysledek skos:Concept
dcterms:description
The thermodynamics of carbon dioxide adsorption in the protonic zeolite H-MCM-22 (Si:Al = 16:1) was investigated by means of adsorption calorimetry and variable-temperature IR spectroscopy, a technique that affords determination of standard adsorption enthalpy (Delta H-0) and entropy (Delta S-0) from analysis of a series of IR spectra recorded over a temperature range while simultaneously measuring equilibrium pressure inside a closed IR cell. Delta H-0 resulted to be -24.5 (+/- 2) kJ mol(-1), while for the entropy change the value of Delta S-0 = -115 (+/- 10) J mol(-1)K(-1) was obtained. The obtained Delta H-0 value is compared with those reported in the literature for the adsorption of CO2 on other zeolites, and discussed in the context of carbon dioxide capture and sequestration. The thermodynamics of carbon dioxide adsorption in the protonic zeolite H-MCM-22 (Si:Al = 16:1) was investigated by means of adsorption calorimetry and variable-temperature IR spectroscopy, a technique that affords determination of standard adsorption enthalpy (Delta H-0) and entropy (Delta S-0) from analysis of a series of IR spectra recorded over a temperature range while simultaneously measuring equilibrium pressure inside a closed IR cell. Delta H-0 resulted to be -24.5 (+/- 2) kJ mol(-1), while for the entropy change the value of Delta S-0 = -115 (+/- 10) J mol(-1)K(-1) was obtained. The obtained Delta H-0 value is compared with those reported in the literature for the adsorption of CO2 on other zeolites, and discussed in the context of carbon dioxide capture and sequestration.
dcterms:title
Combined microcalorimetric and IR spectroscopic study on carbon dioxide adsorption in H-MCM-22 Combined microcalorimetric and IR spectroscopic study on carbon dioxide adsorption in H-MCM-22
skos:prefLabel
Combined microcalorimetric and IR spectroscopic study on carbon dioxide adsorption in H-MCM-22 Combined microcalorimetric and IR spectroscopic study on carbon dioxide adsorption in H-MCM-22
skos:notation
RIV/00216275:25310/14:39898158!RIV15-GA0-25310___
n3:aktivita
n10:P
n3:aktivity
P(GBP106/12/G015)
n3:cisloPeriodika
October
n3:dodaniDat
n7:2015
n3:domaciTvurceVysledku
n14:7420900 n14:9333312
n3:druhVysledku
n11:J
n3:duvernostUdaju
n16:S
n3:entitaPredkladatele
n19:predkladatel
n3:idSjednocenehoVysledku
7813
n3:idVysledku
RIV/00216275:25310/14:39898158
n3:jazykVysledku
n5:eng
n3:klicovaSlova
Zeolites; Thermodynamics; IR spectroscopy; CCS; Carbon dioxide adsorption; Adsorption calorimetry
n3:klicoveSlovo
n6:Thermodynamics n6:IR%20spectroscopy n6:CCS n6:Adsorption%20calorimetry n6:Zeolites n6:Carbon%20dioxide%20adsorption
n3:kodStatuVydavatele
GB - Spojené království Velké Británie a Severního Irska
n3:kontrolniKodProRIV
[8303D9A22969]
n3:nazevZdroje
Applied Surface Science
n3:obor
n13:CF
n3:pocetDomacichTvurcuVysledku
2
n3:pocetTvurcuVysledku
4
n3:projekt
n9:GBP106%2F12%2FG015
n3:rokUplatneniVysledku
n7:2014
n3:svazekPeriodika
316
n3:tvurceVysledku
Bulánek, Roman Delgado, M. R. Arean, C. O. Frolich, Karel
n3:wos
000343329100073
s:issn
0169-4332
s:numberOfPages
5
n17:doi
10.1016/j.apsusc.2014.08.036
n15:organizacniJednotka
25310