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Statements

Subject Item
n2:RIV%2F00216208%3A11320%2F14%3A10289932%21RIV15-MSM-11320___
rdf:type
n4:Vysledek skos:Concept
rdfs:seeAlso
http://dx.doi.org/10.1039/c4fd00051j
dcterms:description
Ultrafast hole dynamics created in molecular systems as a result of sudden ionisation is the focus of much attention in the field of attosecond science. Using the molecule glycine we show through ab initio simulations that the dynamics of a hole, arising from ionisation in the inner valence region, evolves with a timescale appropriate to be measured using X-ray pulses from the current generation of SASE free electron lasers. The examined pump-probe scheme uses X-rays with photon energy below the K edge of carbon (275-280 eV) that will ionise from the inner valence region. A second probe X-ray at the same energy can excite an electron from the core to fill the vacancy in the inner-valence region. The dynamics of the inner valence hole can be tracked by measuring the Auger electrons produced by the subsequent refilling of the core hole as a function of pump-probe delay. We consider the feasibility of the experiment and include numerical simulation to support this analysis. We discuss the potential for all X-ray pump-X-ray probe Auger spectroscopy measurements for tracking hole migration. Ultrafast hole dynamics created in molecular systems as a result of sudden ionisation is the focus of much attention in the field of attosecond science. Using the molecule glycine we show through ab initio simulations that the dynamics of a hole, arising from ionisation in the inner valence region, evolves with a timescale appropriate to be measured using X-ray pulses from the current generation of SASE free electron lasers. The examined pump-probe scheme uses X-rays with photon energy below the K edge of carbon (275-280 eV) that will ionise from the inner valence region. A second probe X-ray at the same energy can excite an electron from the core to fill the vacancy in the inner-valence region. The dynamics of the inner valence hole can be tracked by measuring the Auger electrons produced by the subsequent refilling of the core hole as a function of pump-probe delay. We consider the feasibility of the experiment and include numerical simulation to support this analysis. We discuss the potential for all X-ray pump-X-ray probe Auger spectroscopy measurements for tracking hole migration.
dcterms:title
Analysis of a measurement scheme for ultrafast hole dynamics by few femtosecond resolution X-ray pump-probe Auger spectroscopy Analysis of a measurement scheme for ultrafast hole dynamics by few femtosecond resolution X-ray pump-probe Auger spectroscopy
skos:prefLabel
Analysis of a measurement scheme for ultrafast hole dynamics by few femtosecond resolution X-ray pump-probe Auger spectroscopy Analysis of a measurement scheme for ultrafast hole dynamics by few femtosecond resolution X-ray pump-probe Auger spectroscopy
skos:notation
RIV/00216208:11320/14:10289932!RIV15-MSM-11320___
n3:aktivita
n18:I n18:P
n3:aktivity
I, P(GAP208/12/0521)
n3:cisloPeriodika
April 2014
n3:dodaniDat
n10:2015
n3:domaciTvurceVysledku
n19:8070458
n3:druhVysledku
n17:J
n3:duvernostUdaju
n12:S
n3:entitaPredkladatele
n14:predkladatel
n3:idSjednocenehoVysledku
2613
n3:idVysledku
RIV/00216208:11320/14:10289932
n3:jazykVysledku
n5:eng
n3:klicovaSlova
glycine; amino-acids; vapor-pressures; charge migration
n3:klicoveSlovo
n9:glycine n9:vapor-pressures n9:amino-acids n9:charge%20migration
n3:kodStatuVydavatele
GB - Spojené království Velké Británie a Severního Irska
n3:kontrolniKodProRIV
[8AB333796B71]
n3:nazevZdroje
Faraday Discussions
n3:obor
n13:BE
n3:pocetDomacichTvurcuVysledku
1
n3:pocetTvurcuVysledku
5
n3:projekt
n20:GAP208%2F12%2F0521
n3:rokUplatneniVysledku
n10:2014
n3:svazekPeriodika
171
n3:tvurceVysledku
Cooper, Bridgette Kolorenč, Přemysl Frasinski, Leszek J. Averbukh, Vitali Marangos, Jon P.
n3:wos
000345529900005
s:issn
1359-6640
s:numberOfPages
19
n6:doi
10.1039/c4fd00051j
n16:organizacniJednotka
11320