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Statements

Subject Item
n2:RIV%2F00216208%3A11320%2F13%3A10191396%21RIV14-GA0-11320___
rdf:type
n5:Vysledek skos:Concept
rdfs:seeAlso
http://dx.doi.org/10.1021/jp311978n
dcterms:description
We present results of plasma afterglow experiments on ternary electron ion recombination rate coefficients of H-3(+) and D-3(+) ions at temperatures from 50 to 300 K and compare them to possible three body reaction mechanisms Resonant electron capture into H-3* Rydberg states is likely to be the first step in the ternary recombination, rather than third-body-assisted capture. Subsequent interactions of the Rydberg molecules with ambient neutral and charged particles provide the rate-limiting step that completes the recombination. A semiquantitative model is proposed that reconciles several previously discrepant experimental observations. A rigorous treatment of the problem will require additional theoretical work and experimental investigations. We present results of plasma afterglow experiments on ternary electron ion recombination rate coefficients of H-3(+) and D-3(+) ions at temperatures from 50 to 300 K and compare them to possible three body reaction mechanisms Resonant electron capture into H-3* Rydberg states is likely to be the first step in the ternary recombination, rather than third-body-assisted capture. Subsequent interactions of the Rydberg molecules with ambient neutral and charged particles provide the rate-limiting step that completes the recombination. A semiquantitative model is proposed that reconciles several previously discrepant experimental observations. A rigorous treatment of the problem will require additional theoretical work and experimental investigations.
dcterms:title
Ternary Recombination of H-3(+) and D-3(+) with Electrons in He-H-2 (D-2) Plasmas at Temperatures from 50 to 300 K Ternary Recombination of H-3(+) and D-3(+) with Electrons in He-H-2 (D-2) Plasmas at Temperatures from 50 to 300 K
skos:prefLabel
Ternary Recombination of H-3(+) and D-3(+) with Electrons in He-H-2 (D-2) Plasmas at Temperatures from 50 to 300 K Ternary Recombination of H-3(+) and D-3(+) with Electrons in He-H-2 (D-2) Plasmas at Temperatures from 50 to 300 K
skos:notation
RIV/00216208:11320/13:10191396!RIV14-GA0-11320___
n5:predkladatel
n15:orjk%3A11320
n3:aktivita
n16:S n16:P n16:I
n3:aktivity
I, P(GA205/09/1183), P(GAP209/12/0233), P(OC10046), S
n3:cisloPeriodika
39
n3:dodaniDat
n11:2014
n3:domaciTvurceVysledku
n8:3847632 n8:2913623 n8:8991596 n8:9667334 n8:8133824
n3:druhVysledku
n13:J
n3:duvernostUdaju
n18:S
n3:entitaPredkladatele
n21:predkladatel
n3:idSjednocenehoVysledku
110542
n3:idVysledku
RIV/00216208:11320/13:10191396
n3:jazykVysledku
n14:eng
n3:klicovaSlova
atoms; states; binary; ionization; spectroscopy; afterglow; gas; ions; dissociative recombination; collisional-radiative recombination
n3:klicoveSlovo
n6:binary n6:ionization n6:ions n6:afterglow n6:collisional-radiative%20recombination n6:states n6:atoms n6:spectroscopy n6:gas n6:dissociative%20recombination
n3:kodStatuVydavatele
US - Spojené státy americké
n3:kontrolniKodProRIV
[3C11AD288004]
n3:nazevZdroje
Journal of Physical Chemistry A
n3:obor
n17:BL
n3:pocetDomacichTvurcuVysledku
5
n3:pocetTvurcuVysledku
6
n3:projekt
n4:GAP209%2F12%2F0233 n4:GA205%2F09%2F1183 n4:OC10046
n3:rokUplatneniVysledku
n11:2013
n3:svazekPeriodika
117
n3:tvurceVysledku
Johnsen, R. Plašil, Radek Dohnal, Petr Glosík, Juraj Hejduk, Michal Rubovič, Peter
n3:wos
000326300600019
s:issn
1089-5639
s:numberOfPages
9
n19:doi
10.1021/jp311978n
n9:organizacniJednotka
11320