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Statements

Subject Item
n2:RIV%2F00216208%3A11320%2F12%3A10130860%21RIV13-GA0-11320___
rdf:type
skos:Concept n18:Vysledek
rdfs:seeAlso
http://dx.doi.org/10.1063/1.4730162
dcterms:description
Measurements in H-3(+) afterglow plasmas with spectroscopically determined relative abundances of H-3(+) ions in the para-nuclear and ortho-nuclear spin states provide clear evidence that at low temperatures (77-200 K) para-H-3(+) ions recombine significantly faster with electrons than ions in the ortho state, in agreement with a recent theoretical prediction. The cavity ring-down absorption spectroscopy used here provides an in situ determination of the para/ortho abundance ratio and yields additional information on the translational and rotational temperatures of the recombining ions. The results show that H-3(+) recombination with electrons occurs by both binary recombination and third-body (helium) assisted recombination, and that both the two-body and three-body rate coefficients depend on the nuclear spin states. Electron-stabilized (collisional-radiative) recombination appears to make only a small contribution. (C) 2012 American Institute of Physics. [http://dx.doi.org/10.1063/1.4730162] Measurements in H-3(+) afterglow plasmas with spectroscopically determined relative abundances of H-3(+) ions in the para-nuclear and ortho-nuclear spin states provide clear evidence that at low temperatures (77-200 K) para-H-3(+) ions recombine significantly faster with electrons than ions in the ortho state, in agreement with a recent theoretical prediction. The cavity ring-down absorption spectroscopy used here provides an in situ determination of the para/ortho abundance ratio and yields additional information on the translational and rotational temperatures of the recombining ions. The results show that H-3(+) recombination with electrons occurs by both binary recombination and third-body (helium) assisted recombination, and that both the two-body and three-body rate coefficients depend on the nuclear spin states. Electron-stabilized (collisional-radiative) recombination appears to make only a small contribution. (C) 2012 American Institute of Physics. [http://dx.doi.org/10.1063/1.4730162]
dcterms:title
Binary and ternary recombination of para-H-3(+) and ortho-H-3(+) with electrons: State selective study at 77-200 K Binary and ternary recombination of para-H-3(+) and ortho-H-3(+) with electrons: State selective study at 77-200 K
skos:prefLabel
Binary and ternary recombination of para-H-3(+) and ortho-H-3(+) with electrons: State selective study at 77-200 K Binary and ternary recombination of para-H-3(+) and ortho-H-3(+) with electrons: State selective study at 77-200 K
skos:notation
RIV/00216208:11320/12:10130860!RIV13-GA0-11320___
n18:predkladatel
n19:orjk%3A11320
n3:aktivita
n10:S n10:P
n3:aktivity
P(GA205/09/1183), P(GAP209/12/0233), P(OC10046), S
n3:cisloPeriodika
24
n3:dodaniDat
n17:2013
n3:domaciTvurceVysledku
n7:6787703 n7:6512895 n7:9417559 n7:2913623 n7:8133824 n7:9667334 n7:8991596 n7:3847632
n3:druhVysledku
n6:J
n3:duvernostUdaju
n21:S
n3:entitaPredkladatele
n15:predkladatel
n3:idSjednocenehoVysledku
124954
n3:idVysledku
RIV/00216208:11320/12:10130860
n3:jazykVysledku
n12:eng
n3:klicovaSlova
interstellar; plasmas; afterglow; d-3(+) ions; storage-ring; rate coefficients; h-3(+) ions; dissociative recombination; cavity ringdown spectroscopy; collisional-radiative recombination
n3:klicoveSlovo
n4:rate%20coefficients n4:afterglow n4:cavity%20ringdown%20spectroscopy n4:collisional-radiative%20recombination n4:h-3%28%2B%29%20ions n4:storage-ring n4:plasmas n4:interstellar n4:dissociative%20recombination n4:d-3%28%2B%29%20ions
n3:kodStatuVydavatele
US - Spojené státy americké
n3:kontrolniKodProRIV
[E6E314693E7E]
n3:nazevZdroje
Journal of Chemical Physics
n3:obor
n9:BL
n3:pocetDomacichTvurcuVysledku
8
n3:pocetTvurcuVysledku
9
n3:projekt
n13:GAP209%2F12%2F0233 n13:OC10046 n13:GA205%2F09%2F1183
n3:rokUplatneniVysledku
n17:2012
n3:svazekPeriodika
136
n3:tvurceVysledku
Plašil, Radek Rubovič, Peter Hejduk, Michal Varju, Jozef Roučka, Štěpán Glosík, Juraj Johnsen, Rainer Kotrík, Tomáš Dohnal, Petr
n3:wos
000305881100015
s:issn
0021-9606
s:numberOfPages
14
n16:doi
10.1063/1.4730162
n20:organizacniJednotka
11320