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Statements

Subject Item
n2:RIV%2F00216208%3A11320%2F11%3A10108206%21RIV12-GA0-11320___
rdf:type
skos:Concept n13:Vysledek
rdfs:seeAlso
http://dx.doi.org/10.1002/sia.3717
dcterms:description
Methanol adsorption on ion-sputtered Pt(111) surface exhibiting high concentration of vacancy islands and on (2 x 1) Pt(110) single crystal were investigated by means of photoelectron spectroscopy (PES) and thermal desorption spectroscopy. The measurements showed that methanol adsorbed at low temperature on sputtered Pt(111) and on (2 x 1) Pt(110) surfaces decomposed upon heating. The PES data of methanol adsorption were compared to the data of CO adsorbed on the same Pt single crystal surfaces. In the case of the sputtered Pt(111) surface, the dehydrogenation of H(x)CO intermediates is followed by the CO bond breakage. On the (2 x 1) Pt(110) surface, carbon monoxide, as product of methanol decomposition, desorbed molecularly without appearance of any traces of atomic carbon. By comparing both platinum surfaces we conclude that methanol decomposition occurs at higher temperature on sputtered Pt(111) than on (2 x 1) Pt(110). Copyright (C) 2010 John Wiley & Sons, Ltd. Methanol adsorption on ion-sputtered Pt(111) surface exhibiting high concentration of vacancy islands and on (2 x 1) Pt(110) single crystal were investigated by means of photoelectron spectroscopy (PES) and thermal desorption spectroscopy. The measurements showed that methanol adsorbed at low temperature on sputtered Pt(111) and on (2 x 1) Pt(110) surfaces decomposed upon heating. The PES data of methanol adsorption were compared to the data of CO adsorbed on the same Pt single crystal surfaces. In the case of the sputtered Pt(111) surface, the dehydrogenation of H(x)CO intermediates is followed by the CO bond breakage. On the (2 x 1) Pt(110) surface, carbon monoxide, as product of methanol decomposition, desorbed molecularly without appearance of any traces of atomic carbon. By comparing both platinum surfaces we conclude that methanol decomposition occurs at higher temperature on sputtered Pt(111) than on (2 x 1) Pt(110). Copyright (C) 2010 John Wiley & Sons, Ltd.
dcterms:title
CO and methanol adsorption on (2 x 1)Pt(110) and ion-eroded Pt(111) model catalysts CO and methanol adsorption on (2 x 1)Pt(110) and ion-eroded Pt(111) model catalysts
skos:prefLabel
CO and methanol adsorption on (2 x 1)Pt(110) and ion-eroded Pt(111) model catalysts CO and methanol adsorption on (2 x 1)Pt(110) and ion-eroded Pt(111) model catalysts
skos:notation
RIV/00216208:11320/11:10108206!RIV12-GA0-11320___
n13:predkladatel
n20:orjk%3A11320
n3:aktivita
n12:Z n12:S n12:P
n3:aktivity
P(GD202/09/H041), P(LA08022), P(ME08056), S, Z(MSM0021620834)
n3:cisloPeriodika
10
n3:dodaniDat
n10:2012
n3:domaciTvurceVysledku
n6:1159429 n6:8636303 n6:4473515 Vorokhta, Mykhailo n6:7745214 n6:4895444 n6:2563592
n3:druhVysledku
n19:J
n3:duvernostUdaju
n16:S
n3:entitaPredkladatele
n17:predkladatel
n3:idSjednocenehoVysledku
190696
n3:idVysledku
RIV/00216208:11320/11:10108206
n3:jazykVysledku
n21:eng
n3:klicovaSlova
photoelectron spectroscopy; synchrotron radiation; platinum; CO; methanol
n3:klicoveSlovo
n4:photoelectron%20spectroscopy n4:synchrotron%20radiation n4:CO n4:methanol n4:platinum
n3:kodStatuVydavatele
US - Spojené státy americké
n3:kontrolniKodProRIV
[97C40DE5FFC6]
n3:nazevZdroje
Surface and Interface Analysis
n3:obor
n22:BM
n3:pocetDomacichTvurcuVysledku
7
n3:pocetTvurcuVysledku
9
n3:projekt
n15:LA08022 n15:GD202%2F09%2FH041 n15:ME08056
n3:rokUplatneniVysledku
n10:2011
n3:svazekPeriodika
43
n3:tvurceVysledku
Vorokhta, Mykhailo Johánek, Viktor Skala, T. Škoda, Michal Tsud, Nataliya Matolín, Vladimír Matolínová, Iva Mysliveček, Josef Prince, K. C.
n3:wos
000295450700008
n3:zamer
n11:MSM0021620834
s:issn
0142-2421
s:numberOfPages
7
n9:doi
10.1002/sia.3717
n14:organizacniJednotka
11320