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Statements

Subject Item
n2:RIV%2F00216208%3A11310%2F14%3A10139875%21RIV15-MSM-11310___
rdf:type
skos:Concept n13:Vysledek
rdfs:seeAlso
http://ac.els-cdn.com/S0920586113004173/1-s2.0-S0920586113004173-main.pdf?_tid=e984b2cc-9d66-11e4-9ae4-00000aacb361&acdnat=1421402785_2f5aa15d9f4984d4c8272be48e3c405c
dcterms:description
Surface properties of layered zeolite frameworks, or 2D zeolites, derived from zeolites UTL and ITH are probed by interaction with several small molecules (CH4, CO2, H2O, H2, N2). The dominant feature of the 2D zeolites is the dense grid of the surface silanol groups formed after dissolution of the double 4-member ring building units of the parent 3D zeolites. Compared to the original 3D zeolite frameworks, several distinctive effects contribute to the changes in binding energies: (i) hydrogen-bond and electrostatic interactions with surface silanols, (ii) the confined space effect enhancing dispersion interactions in 3D zeolites and (iii) structural flexibility of 2D zeolites. Surface properties of layered zeolite frameworks, or 2D zeolites, derived from zeolites UTL and ITH are probed by interaction with several small molecules (CH4, CO2, H2O, H2, N2). The dominant feature of the 2D zeolites is the dense grid of the surface silanol groups formed after dissolution of the double 4-member ring building units of the parent 3D zeolites. Compared to the original 3D zeolite frameworks, several distinctive effects contribute to the changes in binding energies: (i) hydrogen-bond and electrostatic interactions with surface silanols, (ii) the confined space effect enhancing dispersion interactions in 3D zeolites and (iii) structural flexibility of 2D zeolites.
dcterms:title
Theoretical investigation of layered zeolite frameworks: Surface properties of 2D zeolites Theoretical investigation of layered zeolite frameworks: Surface properties of 2D zeolites
skos:prefLabel
Theoretical investigation of layered zeolite frameworks: Surface properties of 2D zeolites Theoretical investigation of layered zeolite frameworks: Surface properties of 2D zeolites
skos:notation
RIV/00216208:11310/14:10139875!RIV15-MSM-11310___
n3:aktivita
n20:P n20:I
n3:aktivity
I, P(GBP106/12/G015)
n3:cisloPeriodika
May 2014
n3:dodaniDat
n8:2015
n3:domaciTvurceVysledku
n15:1747681
n3:druhVysledku
n18:J
n3:duvernostUdaju
n6:S
n3:entitaPredkladatele
n17:predkladatel
n3:idSjednocenehoVysledku
50249
n3:idVysledku
RIV/00216208:11310/14:10139875
n3:jazykVysledku
n14:eng
n3:klicovaSlova
2D zeolites; Surface properties; Layered zeolite frameworks
n3:klicoveSlovo
n9:Surface%20properties n9:2D%20zeolites n9:Layered%20zeolite%20frameworks
n3:kodStatuVydavatele
NL - Nizozemsko
n3:kontrolniKodProRIV
[0372B05DB633]
n3:nazevZdroje
Catalysis Today
n3:obor
n19:CF
n3:pocetDomacichTvurcuVysledku
1
n3:pocetTvurcuVysledku
4
n3:projekt
n5:GBP106%2F12%2FG015
n3:rokUplatneniVysledku
n8:2014
n3:svazekPeriodika
227
n3:tvurceVysledku
Hermann, Jan Nachtigall, Petr Bludský, Ota Trachta, Míchal
n3:wos
000332412900002
s:issn
0920-5861
s:numberOfPages
7
n16:doi
10.1016/j.cattod.2013.09.016
n12:organizacniJednotka
11310