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Statements

Subject Item
n2:RIV%2F00216208%3A11310%2F12%3A10132999%21RIV13-MSM-11310___
rdf:type
skos:Concept n15:Vysledek
rdfs:seeAlso
http://dx.doi.org/10.1016/j.chemphys.2012.03.009
dcterms:description
Photogeneration of free charge carriers in poly{1-[4-(trimethylsilyl)phenyl]-2-phenylacetylene} has been studied theoretically. In our work we have utilized our data obtained previously using photoinduced discharge experiment, which showed a steep slope of the dependence of the free charge carriers photogeneration yield on the applied electric field at the low electric field limit, but no saturation plateau. For the theoretical explanation we have utilized our recently developed model (Mensik et al., 2011) [20] that generalizes the model of Arkhipov et al. (2003) [19] by adding an assumption of a resonant reversible coupling of localized excitation to charge transfer states and, consequently, and dependence of internal parameters (permittivity, effective mass of the hole, rate constants) on electric field. Compared to our previous article this work provides a refined analysis of the experimental results on a large variety of intervals of the model parameters. Photogeneration of free charge carriers in poly{1-[4-(trimethylsilyl)phenyl]-2-phenylacetylene} has been studied theoretically. In our work we have utilized our data obtained previously using photoinduced discharge experiment, which showed a steep slope of the dependence of the free charge carriers photogeneration yield on the applied electric field at the low electric field limit, but no saturation plateau. For the theoretical explanation we have utilized our recently developed model (Mensik et al., 2011) [20] that generalizes the model of Arkhipov et al. (2003) [19] by adding an assumption of a resonant reversible coupling of localized excitation to charge transfer states and, consequently, and dependence of internal parameters (permittivity, effective mass of the hole, rate constants) on electric field. Compared to our previous article this work provides a refined analysis of the experimental results on a large variety of intervals of the model parameters.
dcterms:title
Photogeneration of free charge carriers in pi-conjugated polymers with bulky side groups Photogeneration of free charge carriers in pi-conjugated polymers with bulky side groups
skos:prefLabel
Photogeneration of free charge carriers in pi-conjugated polymers with bulky side groups Photogeneration of free charge carriers in pi-conjugated polymers with bulky side groups
skos:notation
RIV/00216208:11310/12:10132999!RIV13-MSM-11310___
n15:predkladatel
n19:orjk%3A11310
n3:aktivita
n9:I n9:P n9:Z
n3:aktivity
I, P(GAP205/10/2280), P(OC10007), Z(AV0Z40500505)
n3:cisloPeriodika
August
n3:dodaniDat
n12:2013
n3:domaciTvurceVysledku
n22:5305993
n3:druhVysledku
n8:J
n3:duvernostUdaju
n14:S
n3:entitaPredkladatele
n18:predkladatel
n3:idSjednocenehoVysledku
158555
n3:idVysledku
RIV/00216208:11310/12:10132999
n3:jazykVysledku
n21:eng
n3:klicovaSlova
localized excitation; charge transfer states; photogeneration of free charge carriers
n3:klicoveSlovo
n5:charge%20transfer%20states n5:photogeneration%20of%20free%20charge%20carriers n5:localized%20excitation
n3:kodStatuVydavatele
NL - Nizozemsko
n3:kontrolniKodProRIV
[2B73B65E406C]
n3:nazevZdroje
Chemical Physics
n3:obor
n7:BM
n3:pocetDomacichTvurcuVysledku
1
n3:pocetTvurcuVysledku
4
n3:projekt
n4:OC10007 n4:GAP205%2F10%2F2280
n3:rokUplatneniVysledku
n12:2012
n3:svazekPeriodika
404
n3:tvurceVysledku
Menšík, M. Pfleger, Jiří Jung, J. Jex, Michal
n3:wos
000308087500010
n3:zamer
n20:AV0Z40500505
s:issn
0301-0104
s:numberOfPages
8
n13:doi
10.1016/j.chemphys.2012.03.009
n16:organizacniJednotka
11310