About: Systematic study of terahertz response of SrTiO3 based heterostructures: Influence of strain, temperature, and electric field     Goto   Sponge   NotDistinct   Permalink

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  • Epitaxial heterostructures consisting of a variable number of SrTiO3/DyScO3 bilayers deposited on DyScO3 substrates were investigated using time-domain terahertz spectroscopy down to helium temperatures. The phase transition into a ferroelectric state is observed in SrTiO3 films in all samples close to 300 K due to in-plane epitaxial strain induced by the substrate and intercalated layers of DyScO3. Evolution of the dielectric spectra with temperature and external electric field is described by a general model which involves a damped harmonic oscillator (soft mode) coupled to a Debye relaxation (central mode). Both modes are connected with the soft mode eigenvector and they reflect a strong anharmonicity of the soft-mode potential. The observed variation of phase transition temperature and of the dielectric response among the structures is ascribed to a partial epitaxial strain relaxation confirmed also by x-ray diffraction.
  • Epitaxial heterostructures consisting of a variable number of SrTiO3/DyScO3 bilayers deposited on DyScO3 substrates were investigated using time-domain terahertz spectroscopy down to helium temperatures. The phase transition into a ferroelectric state is observed in SrTiO3 films in all samples close to 300 K due to in-plane epitaxial strain induced by the substrate and intercalated layers of DyScO3. Evolution of the dielectric spectra with temperature and external electric field is described by a general model which involves a damped harmonic oscillator (soft mode) coupled to a Debye relaxation (central mode). Both modes are connected with the soft mode eigenvector and they reflect a strong anharmonicity of the soft-mode potential. The observed variation of phase transition temperature and of the dielectric response among the structures is ascribed to a partial epitaxial strain relaxation confirmed also by x-ray diffraction. (en)
Title
  • Systematic study of terahertz response of SrTiO3 based heterostructures: Influence of strain, temperature, and electric field
  • Systematic study of terahertz response of SrTiO3 based heterostructures: Influence of strain, temperature, and electric field (en)
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  • Systematic study of terahertz response of SrTiO3 based heterostructures: Influence of strain, temperature, and electric field
  • Systematic study of terahertz response of SrTiO3 based heterostructures: Influence of strain, temperature, and electric field (en)
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  • RIV/68378271:_____/14:00434411!RIV15-GA0-68378271
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  • I, P(GA14-25639S)
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  • RIV/68378271:_____/14:00434411
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  • dielectric response; terahertz spectroscopy; ferroelectrics; thin films; phase transition (en)
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  • US - Spojené státy americké
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  • Physical Review. B
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  • 89
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  • Drahokoupil, Jan
  • Hlinka, Jiří
  • Kužel, Petr
  • Skoromets, Volodymyr
  • Kadlec, Christelle
  • Schubert, J.
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  • 000339048100001
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  • 1098-0121
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  • 10.1103/PhysRevB.89.214116
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