About: Charge transport in TiO2 films with complex percolation pathways investigated by time-resolved terahertz spectroscopy     Goto   Sponge   NotDistinct   Permalink

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  • Depolarization fields play an important role in terahertz experiments on nanostructured samples. Namely, their effects hide peculiarities of nanoscopic charge transport in the spectra measured on these structures. We calculate local fields for percolated and non-percolated model structures by numerical solving of Maxwell equations in the quasi-static limit. The results suggest that in a broad family of structures a simple effective medium approximation model can be applied to characterize the effective response. The model consists in an equivalent circuit composed of a resistance accounting for the percolated chains with an additional parallel RC-branch describing the non-percolated part. We show a recipe for the retrieval of a response connected to the depolarization fields and to the nanoscale transport mechanisms from transient terahertz spectra. Finally, we use the model to interpret our THz photoconductivity spectra in various TiO films with nanofabricated percolation pathways.
  • Depolarization fields play an important role in terahertz experiments on nanostructured samples. Namely, their effects hide peculiarities of nanoscopic charge transport in the spectra measured on these structures. We calculate local fields for percolated and non-percolated model structures by numerical solving of Maxwell equations in the quasi-static limit. The results suggest that in a broad family of structures a simple effective medium approximation model can be applied to characterize the effective response. The model consists in an equivalent circuit composed of a resistance accounting for the percolated chains with an additional parallel RC-branch describing the non-percolated part. We show a recipe for the retrieval of a response connected to the depolarization fields and to the nanoscale transport mechanisms from transient terahertz spectra. Finally, we use the model to interpret our THz photoconductivity spectra in various TiO films with nanofabricated percolation pathways. (en)
Title
  • Charge transport in TiO2 films with complex percolation pathways investigated by time-resolved terahertz spectroscopy
  • Charge transport in TiO2 films with complex percolation pathways investigated by time-resolved terahertz spectroscopy (en)
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  • Charge transport in TiO2 films with complex percolation pathways investigated by time-resolved terahertz spectroscopy
  • Charge transport in TiO2 films with complex percolation pathways investigated by time-resolved terahertz spectroscopy (en)
skos:notation
  • RIV/68378271:_____/13:00393333!RIV14-GA0-68378271
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  • I, P(GA13-12386S), P(GAP204/12/0232)
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  • 3
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  • 65182
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  • RIV/68378271:_____/13:00393333
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  • terahertz spectroscopy; charge transport; TiO2 nanoparticles (en)
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  • US - Spojené státy americké
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  • [B7E9B10055DC]
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  • IEEE Transactions on Terahertz Science and Technology
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  • 3
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  • Fattakhova-Rohlfing, D.
  • Kužel, Petr
  • Mics, Zoltan
  • Němec, Hynek
  • Rychetský, Ivan
  • Bein, T.
  • Mandlmeier, B.
  • Zajac, Vít
http://linked.open...ain/vavai/riv/wos
  • 000318771300012
issn
  • 2156-342X
number of pages
http://bibframe.org/vocab/doi
  • 10.1109/TTHZ.2013.2255555
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