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  • We report on ultrafast photoluminescence (PL) spectroscopy of blue and red-emitting silicon nanostrucures. We prepared samples of porous Si with different dominating PL bands in time-integrated PL spectrum. These samples show also striking differences in ultrafast PL dynamics. For the red-emitting samples we observe rapid PL onset followed by a two-exponential decay, which is spectrally dependent. For the blue-emitting porous Si the PL builds up several ps and decays mono-exponentially with spectrally independent PL rise and decay times. Our results indicate that a dominant part of the blue and red emission comes from two distinct species with different energy states structures. This is also supported by two-photon absorption induced PL measurements. The two-photon and one-photon absorption induced PL spectra, which are identical for the red-emitting samples, differ substantially for the blue-emitting ones.
  • We report on ultrafast photoluminescence (PL) spectroscopy of blue and red-emitting silicon nanostrucures. We prepared samples of porous Si with different dominating PL bands in time-integrated PL spectrum. These samples show also striking differences in ultrafast PL dynamics. For the red-emitting samples we observe rapid PL onset followed by a two-exponential decay, which is spectrally dependent. For the blue-emitting porous Si the PL builds up several ps and decays mono-exponentially with spectrally independent PL rise and decay times. Our results indicate that a dominant part of the blue and red emission comes from two distinct species with different energy states structures. This is also supported by two-photon absorption induced PL measurements. The two-photon and one-photon absorption induced PL spectra, which are identical for the red-emitting samples, differ substantially for the blue-emitting ones. (en)
Title
  • Ultrafast photoluminescence dynamics of blue-emitting silicon nanostructures
  • Ultrafast photoluminescence dynamics of blue-emitting silicon nanostructures (en)
skos:prefLabel
  • Ultrafast photoluminescence dynamics of blue-emitting silicon nanostructures
  • Ultrafast photoluminescence dynamics of blue-emitting silicon nanostructures (en)
skos:notation
  • RIV/68378271:_____/11:00361260!RIV12-AV0-68378271
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  • P(IAA101120804), P(LC510), S, Z(AV0Z10100521), Z(MSM0021620834)
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  • 3
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  • 236660
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  • RIV/68378271:_____/11:00361260
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  • silicon; nanocrystals; time-resolved spectroscopy; luminescence; polarization; two-photon absorption (en)
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  • DE - Spolková republika Německo
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  • [9CD036E1723C]
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  • Physica Status Solidi C: Current Topics in Solid State Physics
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  • 8
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  • Malý, P.
  • Pelant, Ivan
  • Trojánek, F.
  • Gilliot, P.
  • Hönerlange, B.
  • Žídek, K.
http://linked.open...n/vavai/riv/zamer
issn
  • 1862-6351
number of pages
http://bibframe.org/vocab/doi
  • 10.1002/pssc.201000394
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