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  • Optical properties of the cyclic antenna unit LH4 of the bacterial photosystem from purple bacterium Rhodopseudomonas palustris are studied in present paper. Simulated absorption and steady state fluorescence spectra of this molecular system are presented. In addition, localization of exciton states is modeled. The cumulant-expansion method of Mukamel et al. is used for the calculation of spectral responses of the system with exciton-phonon coupling. Dynamic disorder, interaction with a bath, in Markovian approximation simultaneously with two different types of uncorrelated static disorder (the local excitation energy fluctuations and the transfer integral fluctuations) are taking into account in our simulations. For all calculations the software package Mathematica was found very usefull.
  • Optical properties of the cyclic antenna unit LH4 of the bacterial photosystem from purple bacterium Rhodopseudomonas palustris are studied in present paper. Simulated absorption and steady state fluorescence spectra of this molecular system are presented. In addition, localization of exciton states is modeled. The cumulant-expansion method of Mukamel et al. is used for the calculation of spectral responses of the system with exciton-phonon coupling. Dynamic disorder, interaction with a bath, in Markovian approximation simultaneously with two different types of uncorrelated static disorder (the local excitation energy fluctuations and the transfer integral fluctuations) are taking into account in our simulations. For all calculations the software package Mathematica was found very usefull. (en)
Title
  • Intermolecular coupling fluctuation effect on absorption and emission spectra for LH4 ring
  • Intermolecular coupling fluctuation effect on absorption and emission spectra for LH4 ring (en)
skos:prefLabel
  • Intermolecular coupling fluctuation effect on absorption and emission spectra for LH4 ring
  • Intermolecular coupling fluctuation effect on absorption and emission spectra for LH4 ring (en)
skos:notation
  • RIV/62690094:18470/13:50001217!RIV14-MSM-18470___
http://linked.open...avai/predkladatel
http://linked.open...avai/riv/aktivita
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  • I, S
http://linked.open...iv/cisloPeriodika
  • 3
http://linked.open...vai/riv/dodaniDat
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  • 80784
http://linked.open...ai/riv/idVysledku
  • RIV/62690094:18470/13:50001217
http://linked.open...riv/jazykVysledku
http://linked.open.../riv/klicovaSlova
  • Mathematica; localization; exciton states; static and dynamic disorder; absorption spectrum; fluorescence spectrum; LH4; LH2 (en)
http://linked.open.../riv/klicoveSlovo
http://linked.open...odStatuVydavatele
  • US - Spojené státy americké
http://linked.open...ontrolniKodProRIV
  • [E6E0E20DB1F3]
http://linked.open...i/riv/nazevZdroje
  • International journal of mathematics and computers in simulation
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http://linked.open...UplatneniVysledku
http://linked.open...v/svazekPeriodika
  • 7
http://linked.open...iv/tvurceVysledku
  • Heřman, Pavel
  • Zapletal, David
issn
  • 1998-0159
number of pages
http://localhost/t...ganizacniJednotka
  • 18470
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