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  • Recently we determined the iron-partial density of vibrational states (DOS) of nanocrystalline Fe90Zr7B3 (Nanoperm), synthesized by crystallization of an amorphous precursor, for various stages of nanocrystallization separating the DOS of the nanograins from that of the interfaces. Here we present quantitative analysis of the evolution of various thermoelastic properties calculated from DOS such as mean-force constant, mean atomic displacement, vibrational entropy, and lattice specific heat as the material transforms from amorphous, through nanocrystalline, to fully crystallized state. The reported results shed new light on the previously observed anomalies in the vibrational thermodynamics of nanocrystalline materials.
  • Recently we determined the iron-partial density of vibrational states (DOS) of nanocrystalline Fe90Zr7B3 (Nanoperm), synthesized by crystallization of an amorphous precursor, for various stages of nanocrystallization separating the DOS of the nanograins from that of the interfaces. Here we present quantitative analysis of the evolution of various thermoelastic properties calculated from DOS such as mean-force constant, mean atomic displacement, vibrational entropy, and lattice specific heat as the material transforms from amorphous, through nanocrystalline, to fully crystallized state. The reported results shed new light on the previously observed anomalies in the vibrational thermodynamics of nanocrystalline materials. (en)
Title
  • Vibrational thermodynamics of Fe90Zr7B3 nanocrystalline alloy from nuclear inelastic scattering
  • Vibrational thermodynamics of Fe90Zr7B3 nanocrystalline alloy from nuclear inelastic scattering (en)
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  • Vibrational thermodynamics of Fe90Zr7B3 nanocrystalline alloy from nuclear inelastic scattering
  • Vibrational thermodynamics of Fe90Zr7B3 nanocrystalline alloy from nuclear inelastic scattering (en)
skos:notation
  • RIV/61989592:15310/10:10215490!RIV11-MSM-15310___
http://linked.open...avai/riv/aktivita
http://linked.open...avai/riv/aktivity
  • P(1M0512), Z(MSM6198959218)
http://linked.open...iv/cisloPeriodika
  • 14
http://linked.open...vai/riv/dodaniDat
http://linked.open...aciTvurceVysledku
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  • 295638
http://linked.open...ai/riv/idVysledku
  • RIV/61989592:15310/10:10215490
http://linked.open...riv/jazykVysledku
http://linked.open.../riv/klicovaSlova
  • scattering; inelastic; nuclear; alloy; nanocrystalline; Fe90Zr7B3; thermodynamics; Vibrational (en)
http://linked.open.../riv/klicoveSlovo
http://linked.open...odStatuVydavatele
  • US - Spojené státy americké
http://linked.open...ontrolniKodProRIV
  • [C099C79C7AFB]
http://linked.open...i/riv/nazevZdroje
  • Physical Review B (Condensed Matter and Materials Physics)
http://linked.open...in/vavai/riv/obor
http://linked.open...ichTvurcuVysledku
http://linked.open...cetTvurcuVysledku
http://linked.open...vavai/riv/projekt
http://linked.open...UplatneniVysledku
http://linked.open...v/svazekPeriodika
  • 82
http://linked.open...iv/tvurceVysledku
  • Miglierini, Marcel
  • Hu, L.
  • Svec, P.
  • Sergueev, I.
  • Stankov, S.
  • Chumakov, A. I..
  • Rüffer, R.
  • Sepiol, B.
  • Yue, Y. Z..
http://linked.open...ain/vavai/riv/wos
  • 000282507200003
http://linked.open...n/vavai/riv/zamer
issn
  • 1098-0121
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  • 15310
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