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  • Navrhl jsem model založený na klasické teorii nukleace k popisu fázového chování ve stabilní i metastabilní oblasti blízko fázového přechodu prvního řádu. Výsledná stavová rovnice není analytickou funkcí v bodě fázového přechodu. Model jsem otestoval na tekutině tuhých koulí, kde byl zkombinován s viriálovým rozvojem v nízkých hustotách. Neanalytická stavová rovnice je schopna vystihnout %22anomální nárůst%22 tlaku ve vysokých hustotách. Diskutuji důsledky pro popis fázových rovnováh klasickými stavovými rovnicemi. (cs)
  • A model based on classical nucleation theory is proposed to describe phase behavior in stable and metastable regions near a first-order phase transition. The resulting equation of state is not an analytical function at the phase transition point. The model is tested on the hard sphere fluid where it is combined with the virial expansion at low densities. This nonanalytical equation of state is able to capture the observed %22anomalous increase%22 of pressure at high densities. Consequences to description of phase equilibria by classical equations of state are discussed.
  • A model based on classical nucleation theory is proposed to describe phase behavior in stable and metastable regions near a first-order phase transition. The resulting equation of state is not an analytical function at the phase transition point. The model is tested on the hard sphere fluid where it is combined with the virial expansion at low densities. This nonanalytical equation of state is able to capture the observed %22anomalous increase%22 of pressure at high densities. Consequences to description of phase equilibria by classical equations of state are discussed. (en)
Title
  • Nonanalytical equation of state of the hard sphere fluid
  • Neanalytická stavová rovnice tekutiny tuhých koulí (cs)
  • Nonanalytical equation of state of the hard sphere fluid (en)
skos:prefLabel
  • Nonanalytical equation of state of the hard sphere fluid
  • Neanalytická stavová rovnice tekutiny tuhých koulí (cs)
  • Nonanalytical equation of state of the hard sphere fluid (en)
skos:notation
  • RIV/60461373:22340/06:00016724!RIV07-MSM-22340___
http://linked.open.../vavai/riv/strany
  • 464-468
http://linked.open...avai/riv/aktivita
http://linked.open...avai/riv/aktivity
  • P(LC512)
http://linked.open...iv/cisloPeriodika
  • 4
http://linked.open...vai/riv/dodaniDat
http://linked.open...aciTvurceVysledku
http://linked.open.../riv/druhVysledku
http://linked.open...iv/duvernostUdaju
http://linked.open...titaPredkladatele
http://linked.open...dnocenehoVysledku
  • 488790
http://linked.open...ai/riv/idVysledku
  • RIV/60461373:22340/06:00016724
http://linked.open...riv/jazykVysledku
http://linked.open.../riv/klicovaSlova
  • classical nucleation theory; equation of state; hard spheres; nonanalytical function (en)
http://linked.open.../riv/klicoveSlovo
http://linked.open...odStatuVydavatele
  • GB - Spojené království Velké Británie a Severního Irska
http://linked.open...ontrolniKodProRIV
  • [54ADE831BA63]
http://linked.open...i/riv/nazevZdroje
  • Physical Chemistry Chemical Physics
http://linked.open...in/vavai/riv/obor
http://linked.open...ichTvurcuVysledku
http://linked.open...cetTvurcuVysledku
http://linked.open...vavai/riv/projekt
http://linked.open...UplatneniVysledku
http://linked.open...v/svazekPeriodika
  • 8
http://linked.open...iv/tvurceVysledku
  • Kolafa, Jiří
issn
  • 1463-9076
number of pages
http://localhost/t...ganizacniJednotka
  • 22340
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