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  • Ring shaped antenna units of bacterial photosynthetic complexes serve as an ideal models for investigation of the energy transport in real and artificial systems on microscopic level. One has to take into account influence of the environment on the bacteriochlorophyll molecules. Fast fluctuations are simulated by dynamic disorder taken into account using a Markovian treatment of the interaction with the bath. Slow fluctuations are simulated by static disorder here modelled as non-correlated Gaussian disorder in the transfer integrals. One is forced to recalculate every physical quantity (information) for several tausend of different realisations of the static disorder. Progress in computational techniques in recent years allowed effective numerical solution of corresponding dynamic equations of motion. Subsequently the time dependence of the anisotropy of fluorescence after an impulsive excitation in the B800 rings from LH4 complexes of purple bacterium Rhodopseudomonas acidophila is calculated. Th
  • Ring shaped antenna units of bacterial photosynthetic complexes serve as an ideal models for investigation of the energy transport in real and artificial systems on microscopic level. One has to take into account influence of the environment on the bacteriochlorophyll molecules. Fast fluctuations are simulated by dynamic disorder taken into account using a Markovian treatment of the interaction with the bath. Slow fluctuations are simulated by static disorder here modelled as non-correlated Gaussian disorder in the transfer integrals. One is forced to recalculate every physical quantity (information) for several tausend of different realisations of the static disorder. Progress in computational techniques in recent years allowed effective numerical solution of corresponding dynamic equations of motion. Subsequently the time dependence of the anisotropy of fluorescence after an impulsive excitation in the B800 rings from LH4 complexes of purple bacterium Rhodopseudomonas acidophila is calculated. Th (en)
Title
  • Consequences of disorder in ring molecular aggregates: I. Exciton states in single molecule spectroscopy
  • Consequences of disorder in ring molecular aggregates: I. Exciton states in single molecule spectroscopy (en)
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  • Consequences of disorder in ring molecular aggregates: I. Exciton states in single molecule spectroscopy
  • Consequences of disorder in ring molecular aggregates: I. Exciton states in single molecule spectroscopy (en)
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  • RIV/00216275:25410/09:00009097!RIV10-MSM-25410___
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  • 308099
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  • RIV/00216275:25410/09:00009097
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  • molecular ring; exciton states,; tatic and dynamic disorder; anisotropy of fluorescence (en)
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  • [17533C742F38]
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  • Hradec Králové
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  • 16. konference českých a slovenských fyziků 2008
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  • Heřman, Pavel
  • Zapletal, David
  • Barvík, Ivan
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  • 80-86148-93-9
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  • 25410
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