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  • Continental-scale distribution and inter-continental transport of four polychlorinated biphenyl (PCB) congeners (28, 101, 153, 180) from 1950 to 2010 were studied using the global multicompartment chemistry transport model MPI-MCTM. Following identical primary emissions for all PCB congeners into air, most of the burden is stored in terrestrial (soil and vegetation) compartments. Thereby, PCB-28, PCB-101 and PCB-153 show a shift of the soil burden maxima from source to remote regions. This shift is downwind with regard to the westerlies for Eurasia and upwind for North America and more prominent for the lighter PCBs than for PCB-153 or PCB-180. In meridional direction, all congeners' distributions underwent a northward migration in Eurasia and North America since the 1950s. Inter-continental transport from Eurasian sources accounts largely for contamination of Alaska and British Columbia and determines the migration of the PCB distribution in soil in North America.
  • Continental-scale distribution and inter-continental transport of four polychlorinated biphenyl (PCB) congeners (28, 101, 153, 180) from 1950 to 2010 were studied using the global multicompartment chemistry transport model MPI-MCTM. Following identical primary emissions for all PCB congeners into air, most of the burden is stored in terrestrial (soil and vegetation) compartments. Thereby, PCB-28, PCB-101 and PCB-153 show a shift of the soil burden maxima from source to remote regions. This shift is downwind with regard to the westerlies for Eurasia and upwind for North America and more prominent for the lighter PCBs than for PCB-153 or PCB-180. In meridional direction, all congeners' distributions underwent a northward migration in Eurasia and North America since the 1950s. Inter-continental transport from Eurasian sources accounts largely for contamination of Alaska and British Columbia and determines the migration of the PCB distribution in soil in North America. (en)
Title
  • Long-term trends of continental scale PCB patterns studied using a global atmosphere-ocean general circulation model
  • Long-term trends of continental scale PCB patterns studied using a global atmosphere-ocean general circulation model (en)
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  • Long-term trends of continental scale PCB patterns studied using a global atmosphere-ocean general circulation model
  • Long-term trends of continental scale PCB patterns studied using a global atmosphere-ocean general circulation model (en)
skos:notation
  • RIV/00216224:14310/12:00060997!RIV13-MSM-14310___
http://linked.open...avai/predkladatel
http://linked.open...avai/riv/aktivita
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  • P(ED0001/01/01)
http://linked.open...iv/cisloPeriodika
  • 6
http://linked.open...vai/riv/dodaniDat
http://linked.open...aciTvurceVysledku
  • Lammel, Gerhard
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  • 147448
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  • RIV/00216224:14310/12:00060997
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  • Polychlorinated biphenyls; Trans-Pacific transport; Long-range transport; Inter-continental transport; Persistent organic pollutants; Modelling (en)
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  • DE - Spolková republika Německo
http://linked.open...ontrolniKodProRIV
  • [51334FBF5F42]
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  • Environmental Science and Pollution Research
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  • 19
http://linked.open...iv/tvurceVysledku
  • Lammel, Gerhard
  • Stemmler, I.
http://linked.open...ain/vavai/riv/wos
  • 000306123000012
issn
  • 0944-1344
number of pages
http://bibframe.org/vocab/doi
  • 10.1007/s11356-012-0943-8
http://localhost/t...ganizacniJednotka
  • 14310
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