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  • The Heisenberg's uncertainty relation between energy and time restricts our ability to achieve high spectral and temporal resolution in a single experiment, although both are needed to investigate the ultrafast primary processes of photosynthetic light-harvesting. Two distinct experimental concepts providing either spectral or temporal resolution have been developed over the years. We review their basic concepts together with a recent development of new techniques, namely the two-dimensional coherent electronic spectroscopy and the differential fluorescence line-narrowing being applied to the light-harvesting complexes. Extensive collaboration between the Charles University in Prague and the Lund University in Sweden makes it possible to investigate bacterial reaction centers as well as artificial bacteriochlorophyll c aggregates, taking advantages of the both above mentioned techniques. Future prospects for acquiring new knowledge about the recently observed quantum coherence effects in the light-harvesting are discussed.
  • The Heisenberg's uncertainty relation between energy and time restricts our ability to achieve high spectral and temporal resolution in a single experiment, although both are needed to investigate the ultrafast primary processes of photosynthetic light-harvesting. Two distinct experimental concepts providing either spectral or temporal resolution have been developed over the years. We review their basic concepts together with a recent development of new techniques, namely the two-dimensional coherent electronic spectroscopy and the differential fluorescence line-narrowing being applied to the light-harvesting complexes. Extensive collaboration between the Charles University in Prague and the Lund University in Sweden makes it possible to investigate bacterial reaction centers as well as artificial bacteriochlorophyll c aggregates, taking advantages of the both above mentioned techniques. Future prospects for acquiring new knowledge about the recently observed quantum coherence effects in the light-harvesting are discussed. (en)
Title
  • Visualizing Light Harvesting Processes Beyond Heisenberg's Uncertainty
  • Visualizing Light Harvesting Processes Beyond Heisenberg's Uncertainty (en)
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  • Visualizing Light Harvesting Processes Beyond Heisenberg's Uncertainty
  • Visualizing Light Harvesting Processes Beyond Heisenberg's Uncertainty (en)
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  • RIV/00216208:11320/13:10193448!RIV14-GA0-11320___
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  • P(GBP501/12/G055), S
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  • 114218
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  • RIV/00216208:11320/13:10193448
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  • bacteriochlorophyll c aggregates; photosynthetic light harvesting; multidimensional spectroscopy; spectral hole-burning; fluorescence line-narrowing (en)
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  • [627E1F24FC67]
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  • Praha
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  • Praha
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  • WDS'13 Proceedings of Contributed Papers, Part III, Physics
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  • Dědic, Roman
  • Paleček, David
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http://linked.open.../riv/zahajeniAkce
number of pages
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  • MATFYZPRESS
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  • 978-80-7378-252-8
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  • 11320
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