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Description
  • Generalized master equations valid for the third order response of an optically driven multi-level electronic system are derived within Zwanzig projection formalism. Each of three time intervals of the response function is found to require specific master equation and projection operator. Exact cumulant response functions for the harmonic profiles of the potential energy surfaces leading to GAUSSIAN spectral diffusion are reproduced. The proposed method accounts for the nonequilibrium state of bath at the border of intervals, and can be used to improve calculations of ultrafast non-linear spectra of energy transferring systems.
  • Generalized master equations valid for the third order response of an optically driven multi-level electronic system are derived within Zwanzig projection formalism. Each of three time intervals of the response function is found to require specific master equation and projection operator. Exact cumulant response functions for the harmonic profiles of the potential energy surfaces leading to GAUSSIAN spectral diffusion are reproduced. The proposed method accounts for the nonequilibrium state of bath at the border of intervals, and can be used to improve calculations of ultrafast non-linear spectra of energy transferring systems. (en)
Title
  • Quantum master equations for non-linear optical response of molecular systems
  • Quantum master equations for non-linear optical response of molecular systems (en)
skos:prefLabel
  • Quantum master equations for non-linear optical response of molecular systems
  • Quantum master equations for non-linear optical response of molecular systems (en)
skos:notation
  • RIV/00216208:11320/12:10127451!RIV13-GA0-11320___
http://linked.open...avai/predkladatel
http://linked.open...avai/riv/aktivita
http://linked.open...avai/riv/aktivity
  • P(GAP205/10/0989), P(ME 899), Z(MSM0021620835)
http://linked.open...iv/cisloPeriodika
  • 530
http://linked.open...vai/riv/dodaniDat
http://linked.open...aciTvurceVysledku
http://linked.open.../riv/druhVysledku
http://linked.open...iv/duvernostUdaju
http://linked.open...titaPredkladatele
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  • 163826
http://linked.open...ai/riv/idVysledku
  • RIV/00216208:11320/12:10127451
http://linked.open...riv/jazykVysledku
http://linked.open.../riv/klicovaSlova
  • excitons; migration; coherence; temperature; semiconductors; femtosecond spectroscopy (en)
http://linked.open.../riv/klicoveSlovo
http://linked.open...odStatuVydavatele
  • NL - Nizozemsko
http://linked.open...ontrolniKodProRIV
  • [A614BE5458BA]
http://linked.open...i/riv/nazevZdroje
  • Chemical Physics Letters
http://linked.open...in/vavai/riv/obor
http://linked.open...ichTvurcuVysledku
http://linked.open...cetTvurcuVysledku
http://linked.open...vavai/riv/projekt
http://linked.open...UplatneniVysledku
http://linked.open...v/svazekPeriodika
  • 2012
http://linked.open...iv/tvurceVysledku
  • Mančal, Tomáš
  • Šanda, František
http://linked.open...ain/vavai/riv/wos
  • 000301180700026
http://linked.open...n/vavai/riv/zamer
issn
  • 0009-2614
number of pages
http://bibframe.org/vocab/doi
  • 10.1016/j.cplett.2012.01.077
http://localhost/t...ganizacniJednotka
  • 11320
is http://linked.open...avai/riv/vysledek of
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