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  • Exciton spin dynamics in quasi-spherical CdS quantum dots is studied in detail experimentally and theoretically. Exciton states are calculated using the 6-band k?p Hamiltonian. It is shown that for various sets of Luttinger parameters, when the wurtzite lattice crystal field splitting and Coulomb interaction between the electron-hole pair are taken into account exactly, both the electron and hole wavefunction in the lowest exciton state are of S-type. This rules out the spatial-symmetry-induced origin of the dark exciton in CdS quantum dots. The exciton bleaching dynamics is studied using time- and polarization-resolved transient absorption technique of ultrafast laser spectroscopy. Several samples with a different mean size of CdS quantum dots in different glass matrices were investigated. This enabled the separation of effects that are typical for one particular sample from those that are general for this type of material.
  • Exciton spin dynamics in quasi-spherical CdS quantum dots is studied in detail experimentally and theoretically. Exciton states are calculated using the 6-band k?p Hamiltonian. It is shown that for various sets of Luttinger parameters, when the wurtzite lattice crystal field splitting and Coulomb interaction between the electron-hole pair are taken into account exactly, both the electron and hole wavefunction in the lowest exciton state are of S-type. This rules out the spatial-symmetry-induced origin of the dark exciton in CdS quantum dots. The exciton bleaching dynamics is studied using time- and polarization-resolved transient absorption technique of ultrafast laser spectroscopy. Several samples with a different mean size of CdS quantum dots in different glass matrices were investigated. This enabled the separation of effects that are typical for one particular sample from those that are general for this type of material. (en)
Title
  • Exciton spin dynamics in spherical CdS quantum dots
  • Exciton spin dynamics in spherical CdS quantum dots (en)
skos:prefLabel
  • Exciton spin dynamics in spherical CdS quantum dots
  • Exciton spin dynamics in spherical CdS quantum dots (en)
skos:notation
  • RIV/00216208:11320/10:10070136!RIV11-MSM-11320___
http://linked.open...avai/riv/aktivita
http://linked.open...avai/riv/aktivity
  • P(LC510), Z(MSM0021620834)
http://linked.open...iv/cisloPeriodika
  • 4
http://linked.open...vai/riv/dodaniDat
http://linked.open...aciTvurceVysledku
http://linked.open.../riv/druhVysledku
http://linked.open...iv/duvernostUdaju
http://linked.open...titaPredkladatele
http://linked.open...dnocenehoVysledku
  • 258161
http://linked.open...ai/riv/idVysledku
  • RIV/00216208:11320/10:10070136
http://linked.open...riv/jazykVysledku
http://linked.open.../riv/klicovaSlova
  • dots; quantum; CdS; spherical; dynamics; spin; Exciton (en)
http://linked.open.../riv/klicoveSlovo
http://linked.open...odStatuVydavatele
  • US - Spojené státy americké
http://linked.open...ontrolniKodProRIV
  • [281EDBE2C213]
http://linked.open...i/riv/nazevZdroje
  • Physical Review B - Condensed Matter and Materials Physics
http://linked.open...in/vavai/riv/obor
http://linked.open...ichTvurcuVysledku
http://linked.open...cetTvurcuVysledku
http://linked.open...vavai/riv/projekt
http://linked.open...UplatneniVysledku
http://linked.open...v/svazekPeriodika
  • 81
http://linked.open...iv/tvurceVysledku
  • Němec, Petr
  • Malý, Petr
  • Horodyská, Petra
  • Sprinzl, Daniel
  • Devreese, J. T.
  • Gladilin, V. N.
http://linked.open...ain/vavai/riv/wos
  • 000274002500063
http://linked.open...n/vavai/riv/zamer
issn
  • 1098-0121
number of pages
http://localhost/t...ganizacniJednotka
  • 11320
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