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Description
  • The coherent third order optical response of molecular aggregates with fluctuating frequencies, couplings, and transition dipole moments. We derived stochastic nonlinear exciton equations (by combining the quasiparticle picture of excitons with the path integral over stochastic bath paths) and calculated coherent 2D spectra for a tetramer model system whose transition dipole orientations undergo stochastic jumps on an arbitrary timescale. Signatures of domain coherence length fluctuations are observed in the cross peak dynamics in specific pulse polarization configurations.
  • The coherent third order optical response of molecular aggregates with fluctuating frequencies, couplings, and transition dipole moments. We derived stochastic nonlinear exciton equations (by combining the quasiparticle picture of excitons with the path integral over stochastic bath paths) and calculated coherent 2D spectra for a tetramer model system whose transition dipole orientations undergo stochastic jumps on an arbitrary timescale. Signatures of domain coherence length fluctuations are observed in the cross peak dynamics in specific pulse polarization configurations. (en)
Title
  • Exciton Coherence Length Fluctuations in Chromophore Aggregates Probed by Multidimensional Optical Spectroscopy
  • Exciton Coherence Length Fluctuations in Chromophore Aggregates Probed by Multidimensional Optical Spectroscopy (en)
skos:prefLabel
  • Exciton Coherence Length Fluctuations in Chromophore Aggregates Probed by Multidimensional Optical Spectroscopy
  • Exciton Coherence Length Fluctuations in Chromophore Aggregates Probed by Multidimensional Optical Spectroscopy (en)
skos:notation
  • RIV/00216208:11320/10:10061924!RIV11-GA0-11320___
http://linked.open...avai/riv/aktivita
http://linked.open...avai/riv/aktivity
  • P(GP202/07/P245), Z(MSM0021620835)
http://linked.open...iv/cisloPeriodika
  • 1
http://linked.open...vai/riv/dodaniDat
http://linked.open...aciTvurceVysledku
http://linked.open.../riv/druhVysledku
http://linked.open...iv/duvernostUdaju
http://linked.open...titaPredkladatele
http://linked.open...dnocenehoVysledku
  • 258159
http://linked.open...ai/riv/idVysledku
  • RIV/00216208:11320/10:10061924
http://linked.open...riv/jazykVysledku
http://linked.open.../riv/klicovaSlova
  • 2D optical spectroscopy; molecular aggregates; Exciton coherence length (en)
http://linked.open.../riv/klicoveSlovo
http://linked.open...odStatuVydavatele
  • US - Spojené státy americké
http://linked.open...ontrolniKodProRIV
  • [A5C8307249FD]
http://linked.open...i/riv/nazevZdroje
  • Journal of Chemical Physics
http://linked.open...in/vavai/riv/obor
http://linked.open...ichTvurcuVysledku
http://linked.open...cetTvurcuVysledku
http://linked.open...vavai/riv/projekt
http://linked.open...UplatneniVysledku
http://linked.open...v/svazekPeriodika
  • 133
http://linked.open...iv/tvurceVysledku
  • Mukamel, Shaul
  • Šanda, František
  • Perlík, Václav
http://linked.open...ain/vavai/riv/wos
  • 000279640600003
http://linked.open...n/vavai/riv/zamer
issn
  • 0021-9606
number of pages
http://localhost/t...ganizacniJednotka
  • 11320
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