About: Photon energy dependence of graphitization threshold for diamond irradiated with an intense XUV FEL pulse     Goto   Sponge   NotDistinct   Permalink

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  • We studied experimentally and theoretically the structural transition of diamond under an irradiation with an intense femtosecond extreme ultraviolet laser (XUV) pulse of 24–275 eV photon energy provided by free-electron lasers. Experimental results obtained show that the irradiated diamond undergoes a solid-to-solid phase transition to graphite, and not to an amorphous state. Our theoretical findings suggest that the nature of this transition is nonthermal, stimulated by a change of the interatomic potential triggered by the excitation of valence electrons. Ultrashort laser pulse duration enables to identify the subsequent steps of this process: electron excitation, band gap collapse, and the following atomic motion. A good agreement between the experimentally measured and theoretically calculated damage thresholds for the XUV range supports our conclusions.
  • We studied experimentally and theoretically the structural transition of diamond under an irradiation with an intense femtosecond extreme ultraviolet laser (XUV) pulse of 24–275 eV photon energy provided by free-electron lasers. Experimental results obtained show that the irradiated diamond undergoes a solid-to-solid phase transition to graphite, and not to an amorphous state. Our theoretical findings suggest that the nature of this transition is nonthermal, stimulated by a change of the interatomic potential triggered by the excitation of valence electrons. Ultrashort laser pulse duration enables to identify the subsequent steps of this process: electron excitation, band gap collapse, and the following atomic motion. A good agreement between the experimentally measured and theoretically calculated damage thresholds for the XUV range supports our conclusions. (en)
Title
  • Photon energy dependence of graphitization threshold for diamond irradiated with an intense XUV FEL pulse
  • Photon energy dependence of graphitization threshold for diamond irradiated with an intense XUV FEL pulse (en)
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  • Photon energy dependence of graphitization threshold for diamond irradiated with an intense XUV FEL pulse
  • Photon energy dependence of graphitization threshold for diamond irradiated with an intense XUV FEL pulse (en)
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  • RIV/68378271:_____/13:00395857!RIV14-MSM-68378271
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  • I, P(EE2.3.30.0057), P(GA13-28721S), P(GAP108/11/1312), P(GAP205/11/0571), P(GAP208/10/2302), P(LG13029), V
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  • RIV/68378271:_____/13:00395857
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  • graphitization; diamond; XUV; free-electron lase (en)
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  • US - Spojené státy americké
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  • [CF817CB6D6F6]
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  • Physical Review. B
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  • 88
http://linked.open...iv/tvurceVysledku
  • Burian, Tomáš
  • Chalupský, Jaromír
  • Hájková, Věra
  • Juha, Libor
  • Krzywinski, J.
  • Vyšín, Luděk
  • Gaudin, J.
  • Jurek, M.
  • Klinger, D.
  • Sinn, H.
  • Sobierajski, R.
  • Tiedtke, K.
  • Toleikis, S.
  • Tschentscher, T.
  • Wabnitz, H.
  • Vorlíček, Vladimír
  • Toufarová, Martina
  • Saksl, K.
  • Dastjani-Farahani, S.
  • Moeller, S.
  • Harmand, M.
  • Loch, R. A.
  • Nagasono, M.
  • Ozkan, C.
  • Medvedev, N.
  • Jeschke, H. O.
  • Sovák, P.
  • Ziaja, B.
http://linked.open...ain/vavai/riv/wos
  • 000322812700001
issn
  • 1098-0121
number of pages
http://bibframe.org/vocab/doi
  • 10.1103/PhysRevB.88.060101
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