About: d0 ferromagnetic interface between nonmagnetic perovskites     Goto   Sponge   NotDistinct   Permalink

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  • We use computational and experimental methods to study d0 ferromagnetism at a charge-imbalanced interface between two perovskites. In SrTiO3=KTaO3 superlattice calculations, the charge imbalance introduces holes in the SrTiO3 layer, inducing a d0 ferromagnetic half-metallic 2D hole gas at the interface oxygen 2p orbitals. The charge imbalance overrides doping by vacancies at realistic concentrations. Varying the constituent materials shows ferromagnetism to be a general property of hole-type d0 perovskite interfaces. Atomically sharp epitaxial d0 SrTiO3=KTaO3, SrTiO3=KNbO3, and SrTiO3=NaNbO3 interfaces are found to exhibit ferromagnetic hysteresis at room temperature. We suggest that the behavior is due to the high density of states and exchange coupling at the oxygen t1g band in comparison with the more studied d band t2g symmetry electron gas.
  • We use computational and experimental methods to study d0 ferromagnetism at a charge-imbalanced interface between two perovskites. In SrTiO3=KTaO3 superlattice calculations, the charge imbalance introduces holes in the SrTiO3 layer, inducing a d0 ferromagnetic half-metallic 2D hole gas at the interface oxygen 2p orbitals. The charge imbalance overrides doping by vacancies at realistic concentrations. Varying the constituent materials shows ferromagnetism to be a general property of hole-type d0 perovskite interfaces. Atomically sharp epitaxial d0 SrTiO3=KTaO3, SrTiO3=KNbO3, and SrTiO3=NaNbO3 interfaces are found to exhibit ferromagnetic hysteresis at room temperature. We suggest that the behavior is due to the high density of states and exchange coupling at the oxygen t1g band in comparison with the more studied d band t2g symmetry electron gas. (en)
Title
  • d0 ferromagnetic interface between nonmagnetic perovskites
  • d0 ferromagnetic interface between nonmagnetic perovskites (en)
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  • d0 ferromagnetic interface between nonmagnetic perovskites
  • d0 ferromagnetic interface between nonmagnetic perovskites (en)
skos:notation
  • RIV/68378271:_____/12:00390577!RIV15-AV0-68378271
http://linked.open...avai/riv/aktivita
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  • Z(AV0Z10100522)
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  • 12
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  • 132608
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  • RIV/68378271:_____/12:00390577
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  • d0 ferromagnetic interface; perovskite films (en)
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  • US - Spojené státy americké
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  • [D609EEB439A8]
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  • Physical Review Letters
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  • 109
http://linked.open...iv/tvurceVysledku
  • Dejneka, Alexandr
  • Jelínek, Miroslav
  • Kocourek, Tomáš
  • Stupakov, Oleksandr
  • Trepakov, Vladimír
  • Nieminen, R. M.
  • Oja, R.
  • Pinomaa, T.
  • Yao, L.
  • van Dijken, S.
  • Tyunina, Marina
http://linked.open...ain/vavai/riv/wos
  • 000309205500010
http://linked.open...n/vavai/riv/zamer
issn
  • 0031-9007
number of pages
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  • 10.1103/PhysRevLett.109.127207
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