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Description
  • It is important to understand the relative contribution of primary and secondary particles to regional and global aerosol so that models can attribute aerosol radiative forcing to different sources. In large-scale models, there is considerable uncertainty associated with treatments of particle formation (nucleation) in the boundary layer (BL) and in the size distribution of emitted primary particles, leading to uncertainties in predicted cloud condensation nuclei (CCN) concentrations. Here we quantify how primary particle emissions and secondary particle formation influence size-resolved particle number concentrations in the BL using a global aerosol microphysics model and aircraft and ground site observations made during the May 2008 campaign of the EUCAARI. We tested four different parameterisations for BL nucleation and two assumptions for the emission size distribution of anthropogenic and wildfire carbonaceous particles.
  • It is important to understand the relative contribution of primary and secondary particles to regional and global aerosol so that models can attribute aerosol radiative forcing to different sources. In large-scale models, there is considerable uncertainty associated with treatments of particle formation (nucleation) in the boundary layer (BL) and in the size distribution of emitted primary particles, leading to uncertainties in predicted cloud condensation nuclei (CCN) concentrations. Here we quantify how primary particle emissions and secondary particle formation influence size-resolved particle number concentrations in the BL using a global aerosol microphysics model and aircraft and ground site observations made during the May 2008 campaign of the EUCAARI. We tested four different parameterisations for BL nucleation and two assumptions for the emission size distribution of anthropogenic and wildfire carbonaceous particles. (en)
Title
  • Primary Versus Secondary Contributions to Particle Number Concentrations in the European Boundary Layer
  • Primary Versus Secondary Contributions to Particle Number Concentrations in the European Boundary Layer (en)
skos:prefLabel
  • Primary Versus Secondary Contributions to Particle Number Concentrations in the European Boundary Layer
  • Primary Versus Secondary Contributions to Particle Number Concentrations in the European Boundary Layer (en)
skos:notation
  • RIV/67985858:_____/11:00372230!RIV12-AV0-67985858
http://linked.open...avai/riv/aktivita
http://linked.open...avai/riv/aktivity
  • Z(AV0Z40720504)
http://linked.open...iv/cisloPeriodika
  • 23
http://linked.open...vai/riv/dodaniDat
http://linked.open...aciTvurceVysledku
http://linked.open.../riv/druhVysledku
http://linked.open...iv/duvernostUdaju
http://linked.open...titaPredkladatele
http://linked.open...dnocenehoVysledku
  • 223400
http://linked.open...ai/riv/idVysledku
  • RIV/67985858:_____/11:00372230
http://linked.open...riv/jazykVysledku
http://linked.open.../riv/klicovaSlova
  • primary aerosol; secondary aerosol; boundary layer (en)
http://linked.open.../riv/klicoveSlovo
http://linked.open...odStatuVydavatele
  • DE - Spolková republika Německo
http://linked.open...ontrolniKodProRIV
  • [44430F566B56]
http://linked.open...i/riv/nazevZdroje
  • Atmospheric Chemistry and Physics
http://linked.open...in/vavai/riv/obor
http://linked.open...ichTvurcuVysledku
http://linked.open...cetTvurcuVysledku
http://linked.open...UplatneniVysledku
http://linked.open...v/svazekPeriodika
  • 11
http://linked.open...iv/tvurceVysledku
  • Ždímal, Vladimír
  • Zíková, Naděžda
  • Mihalopoulos, N.
  • Kulmala, M.
  • Baltensperger, U.
  • Birmili, W.
  • Flentje, H.
  • Hansson, H.-C.
  • Jennings, S. G.
  • Laj, P.
  • Sellegri, K.
  • Swietlicki, E.
  • Tunved, P.
  • Wiedensohler, A.
  • Aalto, P.
  • Bonasoni, P.
  • Boulon, J.
  • Carslaw, K. S.
  • Coe, H.
  • Collins, L.
  • Duchi, R.
  • Dupuy, R.
  • Frontoso, M. G.
  • Gruening, C.
  • Hamburger, T.
  • Henzing, J. S.
  • Kouvarakis, G.
  • Marinoni, A.
  • Merikanto, J.
  • Minikin, A.
  • Moerman, M.
  • O'Dowd, C. D.
  • Plass-Dülmer, C.
  • Putaund, J.-P.
  • Reddington, C. L.
  • Roldin, P.
  • Sonntag, A.
  • Spracklen, D. V.
  • Tuch, T.
  • Wehner, B.
  • Weingartner, A.
http://linked.open...ain/vavai/riv/wos
  • 000298134300006
http://linked.open...n/vavai/riv/zamer
issn
  • 1680-7316
number of pages
http://bibframe.org/vocab/doi
  • 10.5194/acp-11-12007-2011
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