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Description
  • Intrachain charge carrier transport was studied by means of theoretical computing on the model polymer poly[methyl(phenyl)silylene]. The Marcus theory, in which a dynamic electron-phonon coupling term was inserted into the reorganisation energy, was used for the modelling. The on chain charge carrier mobility was determined as 006 cm2 V1 s1 for 16 mer. For 20 mer, the lower value was found (i.e. 0005 cm2 V1 s1). The experimental value obtained by microwave photoconductivity and time resolved terahertz spectroscopy (pump and probe method) was reported as 002 cm2 V1 s1.
  • Intrachain charge carrier transport was studied by means of theoretical computing on the model polymer poly[methyl(phenyl)silylene]. The Marcus theory, in which a dynamic electron-phonon coupling term was inserted into the reorganisation energy, was used for the modelling. The on chain charge carrier mobility was determined as 006 cm2 V1 s1 for 16 mer. For 20 mer, the lower value was found (i.e. 0005 cm2 V1 s1). The experimental value obtained by microwave photoconductivity and time resolved terahertz spectroscopy (pump and probe method) was reported as 002 cm2 V1 s1. (en)
Title
  • Polaron dynamics in molecular polysilane wires
  • Polaron dynamics in molecular polysilane wires (en)
skos:prefLabel
  • Polaron dynamics in molecular polysilane wires
  • Polaron dynamics in molecular polysilane wires (en)
skos:notation
  • RIV/61389013:_____/11:00371213!RIV12-AV0-61389013
http://linked.open...avai/riv/aktivita
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  • P(KAN400720701), Z(AV0Z40500505)
http://linked.open...iv/cisloPeriodika
  • Suppl. 2
http://linked.open...vai/riv/dodaniDat
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  • 221071
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  • RIV/61389013:_____/11:00371213
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  • Marcus theory; electron-phonon coupling; reorganisation energy (en)
http://linked.open.../riv/klicoveSlovo
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  • GB - Spojené království Velké Británie a Severního Irska
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  • [836143459E65]
http://linked.open...i/riv/nazevZdroje
  • Materials Research Innovations
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  • 15
http://linked.open...iv/tvurceVysledku
  • Nešpůrek, Stanislav
  • Nožár, Juraj
  • Šebera, Jakub
http://linked.open...ain/vavai/riv/wos
  • 000298293300057
http://linked.open...n/vavai/riv/zamer
issn
  • 1432-8917
number of pages
http://bibframe.org/vocab/doi
  • 10.1179/143307511X13031890749451
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