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Description
| - Large-scale plasma was created in molecular gases (CO, CO2, N2, H2O) and their mixtures by high-power laser-induced dielectric breakdown (LIDB). Compositions of the mixtures used are those suggested for the early earth´s atmosphere of neutral and/or mildly reducing character. Time-integrated optical spectra emitted from the laser spark have been measured and analyzed. The spectra of the plasma generated in the CO-containing mixtures are dominated by emission of both C2 and CN radicals. A vibrational temperature of cca 104 K was determined according to an intensity distribution in a vibronic structure of the CN (B2.SIGMA.+.sub/sub.-.SIGMA.+g) violet band. For comparison, the NH3-CH4-H2-H2O mixture has been irradiated as a model of the strongly reducing version of the early earth´s atmosphere. In this mixture, excited CN seems to be significantly less abundant than C2.
- Large-scale plasma was created in molecular gases (CO, CO2, N2, H2O) and their mixtures by high-power laser-induced dielectric breakdown (LIDB). Compositions of the mixtures used are those suggested for the early earth´s atmosphere of neutral and/or mildly reducing character. Time-integrated optical spectra emitted from the laser spark have been measured and analyzed. The spectra of the plasma generated in the CO-containing mixtures are dominated by emission of both C2 and CN radicals. A vibrational temperature of cca 104 K was determined according to an intensity distribution in a vibronic structure of the CN (B2.SIGMA.+.sub/sub.-.SIGMA.+g) violet band. For comparison, the NH3-CH4-H2-H2O mixture has been irradiated as a model of the strongly reducing version of the early earth´s atmosphere. In this mixture, excited CN seems to be significantly less abundant than C2. (en)
- Byla vytvořena plazma v molekulárních plynech (CO, CO2, N2, H2O) a jejich směsích metodou vysoce energetické laserové jiskry. Složení použitých směsí odpovídalo rané atmosféře Země neutrálního a/nebo lehce redukčního charakteru. Byla změřena a analyzována časově nerozlišená spektra záření laserové jiskry. Ve spektrech plasmy, vzniklé ve směsích obsahujících CO, byla dominantní emise C2 a CN radikálů. Vibrační teplota kolem 104 K byla určena z analýzy distribuce intenzit vibronické struktury CN (B2.SIGMA.+.sub/sub.-.SIGMA.+g) pásu v UV oblasti. Pro srovnání byla ozářena směs CH4 - NH3 - N2 - H2O jako příklad silně redukčního typu rané zemské atmosféry. V této směsi byl mnohem menší výskyt excitovaných CN částic než C2. Experimenty s laserovou jiskrou v molekulárních plynech nebyly prováděny pouze ve statickém uspořádání, ale také v plynné trysce (gas-puff target) umístěné ve vakuové interakční komoře. (cs)
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Title
| - Optical and X-ray emission spectroscopy of high-power laser-induced dielectric breakdown in molecular gases and their mixtures
- Optická a rentgenová emisní spektroskopie vysoce energetické laserové jiskry v molekulárních plynech a jejich směsích (cs)
- Optical and X-ray emission spectroscopy of high-power laser-induced dielectric breakdown in molecular gases and their mixtures (en)
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skos:prefLabel
| - Optical and X-ray emission spectroscopy of high-power laser-induced dielectric breakdown in molecular gases and their mixtures
- Optická a rentgenová emisní spektroskopie vysoce energetické laserové jiskry v molekulárních plynech a jejich směsích (cs)
- Optical and X-ray emission spectroscopy of high-power laser-induced dielectric breakdown in molecular gases and their mixtures (en)
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skos:notation
| - RIV/61388955:_____/06:00044414!RIV07-AV0-61388955
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http://linked.open.../vavai/riv/strany
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http://linked.open...avai/riv/aktivita
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http://linked.open...avai/riv/aktivity
| - P(GA203/06/1278), P(LC528), Z(AV0Z10100521), Z(AV0Z40400503), Z(AV0Z40550506)
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http://linked.open...iv/cisloPeriodika
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http://linked.open...vai/riv/dodaniDat
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http://linked.open...aciTvurceVysledku
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http://linked.open.../riv/druhVysledku
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http://linked.open...iv/duvernostUdaju
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http://linked.open...titaPredkladatele
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http://linked.open...dnocenehoVysledku
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http://linked.open...ai/riv/idVysledku
| - RIV/61388955:_____/06:00044414
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http://linked.open...riv/jazykVysledku
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http://linked.open.../riv/klicovaSlova
| - X-ray spectroscopy; LIDB; optical emission spectra (en)
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http://linked.open.../riv/klicoveSlovo
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http://linked.open...odStatuVydavatele
| - US - Spojené státy americké
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http://linked.open...ontrolniKodProRIV
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http://linked.open...i/riv/nazevZdroje
| - Journal of Physical Chemistry. A
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http://linked.open...in/vavai/riv/obor
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http://linked.open...ichTvurcuVysledku
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http://linked.open...cetTvurcuVysledku
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http://linked.open...vavai/riv/projekt
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http://linked.open...UplatneniVysledku
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http://linked.open...v/svazekPeriodika
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http://linked.open...iv/tvurceVysledku
| - Civiš, Svatopluk
- Juha, Libor
- Cihelka, Jaroslav
- Skála, Jiří
- Bittner, Michal
- Pfeifer, Miroslav
- Ryc, L.
- Bartnik, A.
- Fiedorowicz, H.
- Babánková, Dagmar
- Šedivcová, Tereza
- Mikolajczyk, J.
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http://linked.open...n/vavai/riv/zamer
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issn
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number of pages
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