About: Irregular Shapes of Water Clusters Generated in Supersonic Expansions

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rdf:type	skos:Concept http://linked.opendata.cz/ontology/domain/vavai/Vysledek
rdfs:seeAlso	https://journals.aps.org/prl/abstract/10.1103/PhysRevLett.112.113401
Description	We report cross sections for pickup of guest molecules on neutral argon and water clusters with the mean sizes in the range from N=50 to 600. The experiments are supported by molecular dynamics simulations and analytical models based on the interaction potentials. The cross sections for argon clusters are consistent with their assumed spherical shape and follow approximately the theoretically justified N^(1/3) dependence. On the other hand, the cross sections of water clusters depart from this dependence and are considerably larger starting from N?300. We interpret this increase of cross section by the occurrence of highly irregular shapes of water clusters produced in the supersonic expansion of water vapor under the conditions of the large cluster generation. We report cross sections for pickup of guest molecules on neutral argon and water clusters with the mean sizes in the range from N=50 to 600. The experiments are supported by molecular dynamics simulations and analytical models based on the interaction potentials. The cross sections for argon clusters are consistent with their assumed spherical shape and follow approximately the theoretically justified N^(1/3) dependence. On the other hand, the cross sections of water clusters depart from this dependence and are considerably larger starting from N?300. We interpret this increase of cross section by the occurrence of highly irregular shapes of water clusters produced in the supersonic expansion of water vapor under the conditions of the large cluster generation. (en)
Title	Irregular Shapes of Water Clusters Generated in Supersonic Expansions Irregular Shapes of Water Clusters Generated in Supersonic Expansions (en)
skos:prefLabel	Irregular Shapes of Water Clusters Generated in Supersonic Expansions Irregular Shapes of Water Clusters Generated in Supersonic Expansions (en)
skos:notation	RIV/60461373:22340/14:43897827!RIV15-GA0-22340___
http://linked.open...avai/riv/aktivita	I P
http://linked.open...avai/riv/aktivity	I, P(GA14-08937S), P(GAP208/11/0161)
http://linked.open...iv/cisloPeriodika	11
http://linked.open...vai/riv/dodaniDat	2015
http://linked.open...aciTvurceVysledku	Slavíček, Petr
http://linked.open.../riv/druhVysledku	J - Článek v odborném periodiku
http://linked.open...iv/duvernostUdaju	S - Úplné a pravdivé údaje nepodléhající ochraně podle zvláštních právních předpisů
http://linked.open...titaPredkladatele	Vysoká škola chemicko-technologická v Praze / Fakulta chemicko-inženýrská
http://linked.open...dnocenehoVysledku	22869
http://linked.open...ai/riv/idVysledku	RIV/60461373:22340/14:43897827
http://linked.open...riv/jazykVysledku	eng - angličtina
http://linked.open.../riv/klicovaSlova	H2O; GROWTH; CAPTURE; MOBILITY; PARTICLES; MORPHOLOGY; TRANSITION; SIZE; MOLECULAR-BEAM; ATOM SCATTERING (en)
http://linked.open.../riv/klicoveSlovo	SIZE GROWTH PARTICLES ATOM SCATTERING MOLECULAR-BEAM MOBILITY TRANSITION MORPHOLOGY CAPTURE H2O
http://linked.open...odStatuVydavatele	US - Spojené státy americké
http://linked.open...ontrolniKodProRIV	[BBE335F2CF62]
http://linked.open...i/riv/nazevZdroje	Physical Review Letters
http://linked.open...in/vavai/riv/obor	CF
http://linked.open...ichTvurcuVysledku	1 (xsd:int)
http://linked.open...cetTvurcuVysledku	7 (xsd:int)
http://linked.open...vavai/riv/projekt	Dynamicss of Solvated Electrons in Molecular Clusters: Experimental and Theoretical Approach Atmosférické klastry a aerosoly: Experimenty v molekulových paprscích a teorie
http://linked.open...UplatneniVysledku	2014
http://linked.open...v/svazekPeriodika	112
http://linked.open...iv/tvurceVysledku	Fárník, Michal Poterya, Viktoriya Pysanenko, Andriy Slavíček, Petr Fedor, Juraj Lengyel, Jozef Kočišek, Jaroslav
http://linked.open...ain/vavai/riv/wos	000332925900011
issn	0031-9007
number of pages	5 (xsd:int)
http://bibframe.org/vocab/doi	10.1103/PhysRevLett.112.113401
http://localhost/t...ganizacniJednotka	22340

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