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  • The thermodynamics of carbon dioxide adsorption in the protonic zeolite H-MCM-22 (Si:Al = 16:1) was investigated by means of adsorption calorimetry and variable-temperature IR spectroscopy, a technique that affords determination of standard adsorption enthalpy (Delta H-0) and entropy (Delta S-0) from analysis of a series of IR spectra recorded over a temperature range while simultaneously measuring equilibrium pressure inside a closed IR cell. Delta H-0 resulted to be -24.5 (+/- 2) kJ mol(-1), while for the entropy change the value of Delta S-0 = -115 (+/- 10) J mol(-1)K(-1) was obtained. The obtained Delta H-0 value is compared with those reported in the literature for the adsorption of CO2 on other zeolites, and discussed in the context of carbon dioxide capture and sequestration.
  • The thermodynamics of carbon dioxide adsorption in the protonic zeolite H-MCM-22 (Si:Al = 16:1) was investigated by means of adsorption calorimetry and variable-temperature IR spectroscopy, a technique that affords determination of standard adsorption enthalpy (Delta H-0) and entropy (Delta S-0) from analysis of a series of IR spectra recorded over a temperature range while simultaneously measuring equilibrium pressure inside a closed IR cell. Delta H-0 resulted to be -24.5 (+/- 2) kJ mol(-1), while for the entropy change the value of Delta S-0 = -115 (+/- 10) J mol(-1)K(-1) was obtained. The obtained Delta H-0 value is compared with those reported in the literature for the adsorption of CO2 on other zeolites, and discussed in the context of carbon dioxide capture and sequestration. (en)
Title
  • Combined microcalorimetric and IR spectroscopic study on carbon dioxide adsorption in H-MCM-22
  • Combined microcalorimetric and IR spectroscopic study on carbon dioxide adsorption in H-MCM-22 (en)
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  • Combined microcalorimetric and IR spectroscopic study on carbon dioxide adsorption in H-MCM-22
  • Combined microcalorimetric and IR spectroscopic study on carbon dioxide adsorption in H-MCM-22 (en)
skos:notation
  • RIV/00216275:25310/14:39898158!RIV15-GA0-25310___
http://linked.open...avai/riv/aktivita
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  • P(GBP106/12/G015)
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  • October
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  • 7813
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  • RIV/00216275:25310/14:39898158
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  • Zeolites; Thermodynamics; IR spectroscopy; CCS; Carbon dioxide adsorption; Adsorption calorimetry (en)
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  • GB - Spojené království Velké Británie a Severního Irska
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  • [8303D9A22969]
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  • Applied Surface Science
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  • 316
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  • Bulánek, Roman
  • Delgado, M. R.
  • Frolich, Karel
  • Arean, C. O.
http://linked.open...ain/vavai/riv/wos
  • 000343329100073
issn
  • 0169-4332
number of pages
http://bibframe.org/vocab/doi
  • 10.1016/j.apsusc.2014.08.036
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  • 25310
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