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Description
  • A series of new layered coordination polymers consisting of Ln[Ph2P(O)-CH2CH2-P(O)Ph2]1.5 monomeric units, where Ln ) Pr(NO3)3, Nd(NO3)3, NdCl3, Sm(NO3)3, GdCl3, Dy(NO3)3, were synthesized and structurally characterized. The majority of prepared compounds display approximately rectangular building blocks. However, the adopted architecture strongly depends on additional nonbridging ligands in the coordination sphere of the cation, as well as on the reaction conditions and the employed solvent. Accordingly, the solvothermally prepared polymers exhibit either parquet-floor or brick-wall architecture, whereas the polymers from gel-diffusion reactions resemble honeycomb networks. The solvothermal reaction of the smallest lanthanide cation Lu3+ with Ph2P(O)-CH2CH2-P(O)Ph2 led to a molecular compound instead of a polymer.
  • A series of new layered coordination polymers consisting of Ln[Ph2P(O)-CH2CH2-P(O)Ph2]1.5 monomeric units, where Ln ) Pr(NO3)3, Nd(NO3)3, NdCl3, Sm(NO3)3, GdCl3, Dy(NO3)3, were synthesized and structurally characterized. The majority of prepared compounds display approximately rectangular building blocks. However, the adopted architecture strongly depends on additional nonbridging ligands in the coordination sphere of the cation, as well as on the reaction conditions and the employed solvent. Accordingly, the solvothermally prepared polymers exhibit either parquet-floor or brick-wall architecture, whereas the polymers from gel-diffusion reactions resemble honeycomb networks. The solvothermal reaction of the smallest lanthanide cation Lu3+ with Ph2P(O)-CH2CH2-P(O)Ph2 led to a molecular compound instead of a polymer. (en)
Title
  • From Parquets to Bricks: A Series of Lanthanide Coordination Polymers with Bis(diphenylphosphino)ethane Dioxide
  • From Parquets to Bricks: A Series of Lanthanide Coordination Polymers with Bis(diphenylphosphino)ethane Dioxide (en)
skos:prefLabel
  • From Parquets to Bricks: A Series of Lanthanide Coordination Polymers with Bis(diphenylphosphino)ethane Dioxide
  • From Parquets to Bricks: A Series of Lanthanide Coordination Polymers with Bis(diphenylphosphino)ethane Dioxide (en)
skos:notation
  • RIV/00216224:14310/05:00013646!RIV10-MSM-14310___
http://linked.open...avai/riv/aktivita
http://linked.open...avai/riv/aktivity
  • Z(MSM0021622410)
http://linked.open...iv/cisloPeriodika
  • 6
http://linked.open...vai/riv/dodaniDat
http://linked.open...aciTvurceVysledku
http://linked.open.../riv/druhVysledku
http://linked.open...iv/duvernostUdaju
http://linked.open...titaPredkladatele
http://linked.open...dnocenehoVysledku
  • 522168
http://linked.open...ai/riv/idVysledku
  • RIV/00216224:14310/05:00013646
http://linked.open...riv/jazykVysledku
http://linked.open.../riv/klicovaSlova
  • Lanthanides Coordination Polymers (en)
http://linked.open.../riv/klicoveSlovo
http://linked.open...odStatuVydavatele
  • US - Spojené státy americké
http://linked.open...ontrolniKodProRIV
  • [393C66CA368F]
http://linked.open...i/riv/nazevZdroje
  • INORGANIC CHEMISTRY
http://linked.open...in/vavai/riv/obor
http://linked.open...ichTvurcuVysledku
http://linked.open...cetTvurcuVysledku
http://linked.open...UplatneniVysledku
http://linked.open...v/svazekPeriodika
  • 44
http://linked.open...iv/tvurceVysledku
  • Nečas, Marek
  • Pinkas, Jiří
  • Spíchal, Zdeněk
http://linked.open...ain/vavai/riv/wos
  • 000227764700046
http://linked.open...n/vavai/riv/zamer
issn
  • 0020-1669
number of pages
http://localhost/t...ganizacniJednotka
  • 14310
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