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Description
| - Spin and lattice dynamics of CaMn7O12 ceramics were investigated using infrared, THz, and inelastic neutron scattering (INS) spectroscopies in the temperature range 2 to 590 K, and, at low temperatures, in applied magnetic fields of up to 12 T. On cooling, we observed phonon splitting accompanying the structural phase transition at T-C = 450 K as well as the onset of the incommensurately modulated structure at 250 K. In the two antiferromagnetic phases below T-N1 = 90 K and T-N2 = 48 K, several infrared-active excitations emerge in the meV range; their frequencies correspond to the maxima in the magnon density of states obtained by INS. At the magnetic phase transitions, these modes display strong anomalies and, for some of them, a transfer of dielectric strength from the higher-frequency phonons is observed. We propose that these modes are electromagnons. Remarkably, at least two of these modes remain active also in the paramagnetic phase; for this reason, we call them paraelectromagnons. In accordance with this observation, quasielastic neutron scattering revealed short-range magnetic correlations persisting within temperatures up to 500 K above T-N1.
- Spin and lattice dynamics of CaMn7O12 ceramics were investigated using infrared, THz, and inelastic neutron scattering (INS) spectroscopies in the temperature range 2 to 590 K, and, at low temperatures, in applied magnetic fields of up to 12 T. On cooling, we observed phonon splitting accompanying the structural phase transition at T-C = 450 K as well as the onset of the incommensurately modulated structure at 250 K. In the two antiferromagnetic phases below T-N1 = 90 K and T-N2 = 48 K, several infrared-active excitations emerge in the meV range; their frequencies correspond to the maxima in the magnon density of states obtained by INS. At the magnetic phase transitions, these modes display strong anomalies and, for some of them, a transfer of dielectric strength from the higher-frequency phonons is observed. We propose that these modes are electromagnons. Remarkably, at least two of these modes remain active also in the paramagnetic phase; for this reason, we call them paraelectromagnons. In accordance with this observation, quasielastic neutron scattering revealed short-range magnetic correlations persisting within temperatures up to 500 K above T-N1. (en)
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Title
| - Possible coupling between magnons and phonons in multiferroic CaMn7O12
- Possible coupling between magnons and phonons in multiferroic CaMn7O12 (en)
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skos:prefLabel
| - Possible coupling between magnons and phonons in multiferroic CaMn7O12
- Possible coupling between magnons and phonons in multiferroic CaMn7O12 (en)
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skos:notation
| - RIV/00216208:11320/14:10281076!RIV15-MSM-11320___
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http://linked.open...avai/riv/aktivita
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http://linked.open...avai/riv/aktivity
| - I, P(GAP204/12/1163), P(LG11024), P(LM2011025)
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http://linked.open...iv/cisloPeriodika
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http://linked.open...vai/riv/dodaniDat
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http://linked.open...aciTvurceVysledku
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http://linked.open.../riv/druhVysledku
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http://linked.open...iv/duvernostUdaju
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http://linked.open...titaPredkladatele
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http://linked.open...dnocenehoVysledku
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http://linked.open...ai/riv/idVysledku
| - RIV/00216208:11320/14:10281076
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http://linked.open...riv/jazykVysledku
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http://linked.open.../riv/klicovaSlova
| - perovskite; spectroscopy; electromagnons (en)
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http://linked.open.../riv/klicoveSlovo
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http://linked.open...odStatuVydavatele
| - US - Spojené státy americké
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http://linked.open...ontrolniKodProRIV
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http://linked.open...i/riv/nazevZdroje
| - Physical Review B - Condensed Matter and Materials Physics
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http://linked.open...in/vavai/riv/obor
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http://linked.open...ichTvurcuVysledku
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http://linked.open...cetTvurcuVysledku
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http://linked.open...vavai/riv/projekt
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http://linked.open...UplatneniVysledku
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http://linked.open...v/svazekPeriodika
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http://linked.open...iv/tvurceVysledku
| - Kamba, Stanislav
- Kempa, Martin
- Orlita, Milan
- Goian, Veronica
- Kadlec, Christelle
- Kadlec, Filip
- Prokleška, Jan
- Rols, Stephane
- Taylor, Jon
- Vanek, Premysl
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http://linked.open...ain/vavai/riv/wos
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issn
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number of pages
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http://bibframe.org/vocab/doi
| - 10.1103/PhysRevB.90.054307
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http://localhost/t...ganizacniJednotka
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