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  • We report on the femtosecond pump and probe study of the condensation dynamics of electron-hole liquid in CVD IIa type diamond. The parameters of electron-hole liquid created after carrier excitation by one- and two-photon absorption were determined on the basis of die analysis of spectral shape of time-integrated photoluminescence. The dynamics of condensation of carriers into electron-hole liquid was probed by measuring the time evolution of changes in infrared light absorption. These changes were interpreted in terms of the density dependent carrier scattering time according to the Drude model of free-carrier absorption. Measured condensation times range from 50 to 500 ps depending on the initial carrier density (3 x 10(16) cm(-3)-5 x 10(18) cm(-3)) and the sample temperature (13-130 K). The measured dynamics was reproduced very well by a rate equation model of electron-hole droplet formation for low photoexcited carrier densities. A similar to 10 ps delay in initial stage of condensation observed for high carier densities was interpreted in terms of density dependent carrier cooling rate.
  • We report on the femtosecond pump and probe study of the condensation dynamics of electron-hole liquid in CVD IIa type diamond. The parameters of electron-hole liquid created after carrier excitation by one- and two-photon absorption were determined on the basis of die analysis of spectral shape of time-integrated photoluminescence. The dynamics of condensation of carriers into electron-hole liquid was probed by measuring the time evolution of changes in infrared light absorption. These changes were interpreted in terms of the density dependent carrier scattering time according to the Drude model of free-carrier absorption. Measured condensation times range from 50 to 500 ps depending on the initial carrier density (3 x 10(16) cm(-3)-5 x 10(18) cm(-3)) and the sample temperature (13-130 K). The measured dynamics was reproduced very well by a rate equation model of electron-hole droplet formation for low photoexcited carrier densities. A similar to 10 ps delay in initial stage of condensation observed for high carier densities was interpreted in terms of density dependent carrier cooling rate. (en)
Title
  • Dynamics of electron-hole liquid condensation in CVD diamond studied by femtosecond pump and probe spectroscopy
  • Dynamics of electron-hole liquid condensation in CVD diamond studied by femtosecond pump and probe spectroscopy (en)
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  • Dynamics of electron-hole liquid condensation in CVD diamond studied by femtosecond pump and probe spectroscopy
  • Dynamics of electron-hole liquid condensation in CVD diamond studied by femtosecond pump and probe spectroscopy (en)
skos:notation
  • RIV/00216208:11320/13:10173366!RIV14-GA0-11320___
http://linked.open...avai/riv/aktivita
http://linked.open...avai/riv/aktivity
  • P(GD202/09/H041), S
http://linked.open...iv/cisloPeriodika
  • January 2013
http://linked.open...vai/riv/dodaniDat
http://linked.open...aciTvurceVysledku
http://linked.open.../riv/druhVysledku
http://linked.open...iv/duvernostUdaju
http://linked.open...titaPredkladatele
http://linked.open...dnocenehoVysledku
  • 70960
http://linked.open...ai/riv/idVysledku
  • RIV/00216208:11320/13:10173366
http://linked.open...riv/jazykVysledku
http://linked.open.../riv/klicovaSlova
  • Phase transition; Optical high excitation of diamond; Pump and probe spectroscopy; Electron-hole liquid (en)
http://linked.open.../riv/klicoveSlovo
http://linked.open...odStatuVydavatele
  • NL - Nizozemsko
http://linked.open...ontrolniKodProRIV
  • [8C68ADBEFB79]
http://linked.open...i/riv/nazevZdroje
  • Diamond and Related Materials
http://linked.open...in/vavai/riv/obor
http://linked.open...ichTvurcuVysledku
http://linked.open...cetTvurcuVysledku
http://linked.open...vavai/riv/projekt
http://linked.open...UplatneniVysledku
http://linked.open...v/svazekPeriodika
  • 34
http://linked.open...iv/tvurceVysledku
  • Malý, Petr
  • Kozák, Martin
  • Trojánek, František
  • Popelář, Tomáš
http://linked.open...ain/vavai/riv/wos
  • 000317795400003
issn
  • 0925-9635
number of pages
http://bibframe.org/vocab/doi
  • 10.1016/j.diamond.2013.01.008
http://localhost/t...ganizacniJednotka
  • 11320
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