About: Organized Mesoporous TiO2 Films Stabilized by Phosphorus: Application for Dye-Sensitized Solar Cells

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rdf:type	skos:Concept http://linked.opendata.cz/ontology/domain/vavai/Vysledek
Description	A synthetic protocol was developed for the preparation of thin mesoporous TiO2 films with enhanced thermal stability. This objective was achieved by a modification of the procedure of supramolecular templating by a Pluronic P-123 copolymer by an addition of a small amount of phosphoric acid to the precursor solution. Thin mesoporous TiO2 films up to 2.3 µm thick were prepared via layer-by-layer deposition. The roughness factor exceeding 1300 was achieved on these films. After annealing at 540°C, well-developed 5–6 nm anatase nanocrystals were present in the pore walls of a still perfect mesoporous structure. The pore coalescence and structure collapse during heat-treatment were effectively hindered by the presence of phosphorus. Our P-modified mesoporous TiO2 films were sensitized with the N-945 dye and used as photoanodes of the dye-sensitized solar cells. They reached the conversion efficiency of 5.03 or 5.05% for the film thickness of 1.8 or 2.3 µm, respectively. A synthetic protocol was developed for the preparation of thin mesoporous TiO2 films with enhanced thermal stability. This objective was achieved by a modification of the procedure of supramolecular templating by a Pluronic P-123 copolymer by an addition of a small amount of phosphoric acid to the precursor solution. Thin mesoporous TiO2 films up to 2.3 µm thick were prepared via layer-by-layer deposition. The roughness factor exceeding 1300 was achieved on these films. After annealing at 540°C, well-developed 5–6 nm anatase nanocrystals were present in the pore walls of a still perfect mesoporous structure. The pore coalescence and structure collapse during heat-treatment were effectively hindered by the presence of phosphorus. Our P-modified mesoporous TiO2 films were sensitized with the N-945 dye and used as photoanodes of the dye-sensitized solar cells. They reached the conversion efficiency of 5.03 or 5.05% for the film thickness of 1.8 or 2.3 µm, respectively. (en)
Title	Organized Mesoporous TiO2 Films Stabilized by Phosphorus: Application for Dye-Sensitized Solar Cells Organized Mesoporous TiO2 Films Stabilized by Phosphorus: Application for Dye-Sensitized Solar Cells (en)
skos:prefLabel	Organized Mesoporous TiO2 Films Stabilized by Phosphorus: Application for Dye-Sensitized Solar Cells Organized Mesoporous TiO2 Films Stabilized by Phosphorus: Application for Dye-Sensitized Solar Cells (en)
skos:notation	RIV/61388955:_____/10:00331908!RIV11-MSM-61388955
http://linked.open...avai/riv/aktivita	P Z
http://linked.open...avai/riv/aktivity	P(IAA400400804), P(KAN100500652), P(KAN200100801), P(LC510), P(OC09048), Z(AV0Z40400503)
http://linked.open...iv/cisloPeriodika	1
http://linked.open...vai/riv/dodaniDat	2011
http://linked.open...aciTvurceVysledku	Zukalová, Markéta Kavan, Ladislav Zukal, Arnošt Procházka, Jan
http://linked.open.../riv/druhVysledku	J - Článek v odborném periodiku
http://linked.open...iv/duvernostUdaju	S - Úplné a pravdivé údaje nepodléhající ochraně podle zvláštních právních předpisů
http://linked.open...titaPredkladatele	Ústav fyzikální chemie J. Heyrovského AV ČR, v.v.i.
http://linked.open...dnocenehoVysledku	277516
http://linked.open...ai/riv/idVysledku	RIV/61388955:_____/10:00331908
http://linked.open...riv/jazykVysledku	eng - angličtina
http://linked.open.../riv/klicovaSlova	annealing; anodes; mesoporous materials; dyes (en)
http://linked.open.../riv/klicoveSlovo	mesoporous materials annealing dyes anodes
http://linked.open...odStatuVydavatele	US - Spojené státy americké
http://linked.open...ontrolniKodProRIV	[0E8FD8A82FD5]
http://linked.open...i/riv/nazevZdroje	Journal of the Electrochemical Society
http://linked.open...in/vavai/riv/obor	CG
http://linked.open...ichTvurcuVysledku	4 (xsd:int)
http://linked.open...cetTvurcuVysledku	6 (xsd:int)
http://linked.open...vavai/riv/projekt	Center of nanotechnology and materials for nanoelectronics Supramolecular assemblies with carbon nanotubes Heterogeneous and hybrid nanocomposite materials for solar cells Bioactive Biocompatible Surfaces and Novel Nanostructured Composites for Applications to Medicine and Drug Delivery Nanocrystalline oxidic semiconductors for optoelectronic applications
http://linked.open...UplatneniVysledku	2010
http://linked.open...v/svazekPeriodika	157
http://linked.open...iv/tvurceVysledku	Kavan, Ladislav Zukalová, Markéta Zukal, Arnošt Procházka, Jan Yum, J. H. Graetzel, M.
http://linked.open...ain/vavai/riv/wos	000272387200094
http://linked.open...n/vavai/riv/zamer	Struktura, reaktivita a dynamika molekulárních a biomolekulárních systémů: teorie, experiment, aplikace
issn	0013-4651
number of pages	5 (xsd:int)
is http://linked.open...avai/riv/vysledek of	Organized Mesoporous TiO2 Films Stabilized by Phosphorus: Application for Dye-Sensitized Solar Cells Organized Mesoporous TiO2 Films Stabilized by Phosphorus: Application for Dye-Sensitized Solar Cells Organized Mesoporous TiO2 Films Stabilized by Phosphorus: Application for Dye-Sensitized Solar Cells

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