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  • The magnetic phase transitions for Gd(0 0 0 1) grown on W(1 1 0) – a bulk transition at 293 K and a surface transition about 85 K above this – are found to influence the energy separation of the Gd 5s and 4s core-photoelectron doublets. The 5s doublet separation ΔE5s changes over a range of temperatures spanning these transitions, and decreases by a maximum of 60 meV in this region, but then recovers its original value; the 4s doublet shows a smaller change in the reverse direction, which does not recover at high temperature. Some of these effects are semi-quantitatively understood from free-atom multiplet theory and from theoretical calculations based on all-electron LDA+U calculations including 4f electron correlation effects.
  • The magnetic phase transitions for Gd(0 0 0 1) grown on W(1 1 0) – a bulk transition at 293 K and a surface transition about 85 K above this – are found to influence the energy separation of the Gd 5s and 4s core-photoelectron doublets. The 5s doublet separation ΔE5s changes over a range of temperatures spanning these transitions, and decreases by a maximum of 60 meV in this region, but then recovers its original value; the 4s doublet shows a smaller change in the reverse direction, which does not recover at high temperature. Some of these effects are semi-quantitatively understood from free-atom multiplet theory and from theoretical calculations based on all-electron LDA+U calculations including 4f electron correlation effects. (en)
Title
  • Observation of dynamical spin-dependent electron interactions and screening in magnetic transitions via core-level multiplet-energy separations
  • Observation of dynamical spin-dependent electron interactions and screening in magnetic transitions via core-level multiplet-energy separations (en)
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  • Observation of dynamical spin-dependent electron interactions and screening in magnetic transitions via core-level multiplet-energy separations
  • Observation of dynamical spin-dependent electron interactions and screening in magnetic transitions via core-level multiplet-energy separations (en)
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  • RIV/68378271:_____/13:00424501!RIV14-AV0-68378271
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  • 93001
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  • RIV/68378271:_____/13:00424501
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  • photoelectron spectroscopy; electronic structure (en)
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  • NL - Nizozemsko
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  • Journal of Electron Spectroscopy and Related Phenomena
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  • 189
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  • Shick, Alexander
  • Denecke, R.
  • Fadley, C. S.
  • Hussain, Z.
  • Liesegang, J.
  • Morais, J.
  • Palomares, F. J.
  • Pickett, W. E.
  • Tober, E. D.
  • Ynzunza, R.X.
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  • 000329423000026
issn
  • 0368-2048
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  • 10.1016/j.elspec.2012.12.009
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